Levels and distribution of heavy metals in atmospheric particular matters over the northern South China Sea

被引:5
作者
Xu, Weihai [1 ]
Yan, Wen [1 ]
Zhang, Gan [2 ]
Li, Jun [2 ]
Miao, Li [1 ]
Huang, Weixia [1 ]
机构
[1] Chinese Acad Sci, South China Sea Inst Oceanol, CAS Key Lab Marginal Sea Geol, Guangzhou 510301, Guangdong, Peoples R China
[2] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
关键词
South China Sea; Heavymetals; Asian monsoon; Atmospheric transport; LONG-RANGE TRANSPORT; TRACE-METALS; CHEMICAL-COMPOSITION; LEADED GASOLINE; AEROSOL; AIR; COASTAL; DEPOSITION; ATLANTIC; ELEMENTS;
D O I
10.1007/s11356-014-2810-2
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Oceans play a significant role in the cycling of trace metals and persistent organic pollutants. In this study, aerosol samples covering the whole northern South China Sea (SCS) were collected in 2005 and 2007, respectively, for analysis of trace metals and major elements. The levels of trace metals detected ranged from 0.514 to 119 ng/m(3) in 2005 and from 0.130 to 24.2 ng/m(3) in 2007, respectively. Cu, Zn, and Pb were the three predominant metals with high enrichment factors (> 10), indicating the strong anthropogenic inputs. The trace metals over SCS were comparable to the values in suburban and background sites of South China, but generally higher than those over other seas and oceans. Considering the fact that they were influenced by their proximity to source regions and air mass origins, the elevated metals in 2005 were probably attributed to the strong wind and long-range atmospheric transport driven by Asian monsoon.
引用
收藏
页码:8774 / 8781
页数:8
相关论文
共 42 条
[1]   Equatorward expansion of the westward electrojet during magnetically disturbed periods [J].
Ahn, BH ;
Chen, GX ;
Sun, W ;
Gjerloev, JW ;
Kamide, Y ;
Sigwarth, JB ;
Frank, LA .
JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS, 2005, 110 (A1)
[2]  
[Anonymous], J GEOPHYS RES
[3]   Mercury in particulate matter over Polish zone of the southern Baltic Sea [J].
Beldowska, M. ;
Saniewska, D. ;
Falkowska, L. ;
Lewandowska, A. .
ATMOSPHERIC ENVIRONMENT, 2012, 46 :397-404
[4]   Heavy metal deposition fluxes affecting an Atlantic coastal area in the southwest of Spain [J].
Castillo, Sonia ;
de la Rosa, Jesus D. ;
Sanchez de la Campa, Ana M. ;
Gonzalez-Castanedo, Yolanda ;
Fernandez-Camacho, Rocio .
ATMOSPHERIC ENVIRONMENT, 2013, 77 :509-517
[5]   Trace metal chemistry of particulate aerosols from the UK mainland coastal rim of the NE Irish sea [J].
Chester, R ;
Nimmo, M ;
Fones, GR ;
Keyse, S ;
Zhang, Z .
ATMOSPHERIC ENVIRONMENT, 2000, 34 (06) :949-958
[6]   THE WET DEPOSITION OF TRACE-METALS TO THE WESTERN ATLANTIC OCEAN AT THE MID-ATLANTIC COAST AND ON BERMUDA [J].
CHURCH, TM ;
TRAMONTANO, JM ;
SCUDLARK, JR ;
JICKELLS, TD ;
TOKOS, JJ ;
KNAP, AH ;
GALLOWAY, JN .
ATMOSPHERIC ENVIRONMENT, 1984, 18 (12) :2657-2664
[7]   Elemental composition of aerosol in the Nam Co region, Tibetan Plateau, during summer monsoon season [J].
Cong, Zhiyuan ;
Kang, Shichang ;
Liu, Xiande ;
Wang, Guangfu .
ATMOSPHERIC ENVIRONMENT, 2007, 41 (06) :1180-1187
[8]   Atmospheric aerosol concentration level and chemical characteristics of water-soluble ionic species in wintertime in Beijing, China [J].
Duan, FK ;
Liu, XD ;
He, KB ;
Lu, YQ ;
Wang, L .
JOURNAL OF ENVIRONMENTAL MONITORING, 2003, 5 (04) :569-573
[9]   Characterization of particulate, metallic elements of TSP, PM2.5 and PM2.5-10 aerosols at a farm sampling site in Taiwan, Taichung [J].
Fang, GC ;
Chang, CN ;
Chu, CC ;
Wu, YS ;
Fu, PPC ;
Yang, IL ;
Chen, MH .
SCIENCE OF THE TOTAL ENVIRONMENT, 2003, 308 (1-3) :157-166
[10]   Seasonality of major aerosol species and their transformations in Cairo megacity [J].
Favez, Olivier ;
Cachler, Helene ;
Sciare, Jean ;
Alfaro, Stephane C. ;
El-Araby, Tarek M. ;
Harhash, Maha A. ;
Abdelwahab, Magdy M. .
ATMOSPHERIC ENVIRONMENT, 2008, 42 (07) :1503-1516