Adsorption of aniline from aqueous solution using graphene oxide-modified attapulgite composites

被引:33
作者
Deng, Qiulin [1 ,2 ]
Chen, Chong [1 ]
Lei, Qin [1 ]
Liang, Jianhao [1 ]
Zhang, Tinghong [1 ]
Jiang, Jinlong [2 ]
机构
[1] Southwest Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Environm Friendly Energy Mat, 59 Qinglong Rd, Mianyang 621010, Peoples R China
[2] Huaiyin Inst Technol, Jiangsu Prov Key Lab Palygorskite Sci & Appl Tech, 1 Meicheng Rd, Huaian 223003, Peoples R China
来源
RSC ADVANCES | 2018年 / 8卷 / 41期
关键词
METHYLENE-BLUE DYE; METAL-IONS; REMOVAL; CARBON; NANOCOMPOSITE; PHENOL; POLLUTANTS; ADSORBENT; NITRIDE; U(VI);
D O I
10.1039/c8ra04143a
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Adsorption is an efficient treatment method for aniline removal in water treatment. In this work, the composites of graphene oxide-modified attapulgite were prepared and used firstly to remove aniline from wastewater. The composites were characterized by Fourier transformed infrared, Brunauer-Emmett-Teller, scanning electron microscopy and X-ray diffraction analysis. The effects of initial concentration, time, temperature and pH value on adsorption of aniline on graphene oxide-modified attapulgite are investigated. pH and temperature are found to have a significant influence on the adsorption amount. The experimental results showed that graphene oxide-modified attapulgite possesses strong adsorption ability for aniline with hydrogen bond interaction. The saturated adsorption amount could reach up to 90 mg g(-1) at pH = 2-4. The Langmuir isotherm is found to describe well the equilibrium adsorption data. Finally, graphene oxide-modified attapulgite is also observed to possess excellent reusability.
引用
收藏
页码:23382 / 23389
页数:8
相关论文
共 48 条
[1]  
Aljeboree AM, 2015, RES J PHARM BIOL CHE, V6, P778
[2]   Adsorption of aniline from aqueous solution using novel adsorbent PAM/SiO2 [J].
An, Fuqiang ;
Feng, Xiaoqin ;
Gao, Baojiao .
CHEMICAL ENGINEERING JOURNAL, 2009, 151 (1-3) :183-187
[3]  
[Anonymous], 1996, Integrated Wastewater Discharge Standard. Ministry of Environmental Protection of the People's Republic of China: Beijing
[4]   Effect of hydrogen peroxide on aniline oxidation by electro-Fenton and fluidized-bed Fenton processes [J].
Anotai, Jin ;
Su, Chia-Chi ;
Tsai, Yi-Chun ;
Lu, Ming-Chun .
JOURNAL OF HAZARDOUS MATERIALS, 2010, 183 (1-3) :888-893
[5]   Adsorption of graphene for the removal of inorganic pollutants in water purification: a review [J].
Cao, Yong ;
Li, Xinbao .
ADSORPTION-JOURNAL OF THE INTERNATIONAL ADSORPTION SOCIETY, 2014, 20 (5-6) :713-727
[6]   Adsorption study for removal of Congo red anionic dye using organo-attapulgite [J].
Chen, H. ;
Zhao, J. .
ADSORPTION-JOURNAL OF THE INTERNATIONAL ADSORPTION SOCIETY, 2009, 15 (04) :381-389
[7]   Synthesis of an Attapulgite Clay@Carbon Nanocomposite Adsorbent by a Hydrothermal Carbonization Process and Their Application in the Removal of Toxic Metal Ions from Water [J].
Chen, Li-Feng ;
Lang, Hai-Wei ;
Lu, Yang ;
Cui, Chun-Hua ;
Yu, Shu-Hong .
LANGMUIR, 2011, 27 (14) :8998-9004
[8]   A Copper(II)-Paddlewheel Metal-Organic Framework with Exceptional Hydrolytic Stability and Selective Adsorption and Detection Ability of Aniline in Water [J].
Chen, Ya ;
Wang, Bin ;
Wang, Xiaoqing ;
Xie, Lin-Hua ;
Li, Jinping ;
Xie, Yabo ;
Li, Jian-Rong .
ACS APPLIED MATERIALS & INTERFACES, 2017, 9 (32) :27027-27035
[9]   RETRACTED: Mutual effect of U(VI) and Sr(II) on graphene oxides: evidence from EXAFS and theoretical calculations (Retracted article. See vol. 7, pg. 1617, 2020) [J].
Cheng, Wencai ;
Ding, Congcong ;
Wu, Qunyan ;
Wang, Xiangxue ;
Sun, Yubing ;
Shi, Weiqun ;
Hayat, Tasawar ;
Alsaedi, Ahmed ;
Chai, Zhifang ;
Wang, Xiangke .
ENVIRONMENTAL SCIENCE-NANO, 2017, 4 (05) :1124-1131
[10]   The effect of solution pH and peroxide in the TiO2-induced photocatalysis of chlorinated aniline [J].
Chu, W. ;
Choy, W. K. ;
So, T. Y. .
JOURNAL OF HAZARDOUS MATERIALS, 2007, 141 (01) :86-91