A historical record of the impact of nuclear activities based on 129I in coral cores in Baler, Philippines: An update

被引:7
|
作者
Bautista, Angel T. [1 ]
Limlingan, Sophia Jobien M. [1 ]
Bauyon, Mary Margareth T. [1 ]
Jagonoy, Arvin M. [1 ]
Racho, Joseph Michael D. [1 ]
Valdez, Jeff Darren G. [1 ]
Salon, Jay T. [2 ]
Tabuso, Aldrin Jan E. [2 ]
Valerio, John Kenneth C. [2 ]
Dumalagan, Edwin E., Jr. [3 ]
Kusuno, Haruka [4 ]
Siringan, Fernando P. [3 ]
Matsuzaki, Hiroyuki [4 ]
机构
[1] Philippine Nucl Res Inst, Dept Sci & Technol DOST PNRI, Commonwealth Ave, Quezon City 1101, Philippines
[2] Ind Technol Dev Inst, Adv Device & Mat Testing Lab ITDI ADMATEL, DOST Compound, Gen Santos Ave, Taguig City 1631, Philippines
[3] Univ Philippines Diliman, Marine Sci Inst, Quezon City 1101, Philippines
[4] Univ Tokyo, Univ Museum, Micro Anal Lab, Tandem Accelerator MALT,Bunkyo Ku, 2-11-16 Yayoi, Tokyo 1130032, Japan
关键词
Iodine-129; Nuclear weapons; Nuclear fuel reprocessing; Nuclear accident; Accelerator mass spectrometry; SEA-SURFACE TEMPERATURE; IODINE ISOTOPES; FUKUSHIMA; OCEAN; RADIOCARBON; DEPOSITION; KUROSHIO; AMS;
D O I
10.1016/j.jenvrad.2020.106508
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In a previous study in 2016, we presented how I-129 in coral cores from the east (Baler) and west (Parola) sides of the Philippines recorded the impacts of human nuclear activities, including nuclear weapons testing, nuclear fuel reprocessing, and nuclear accidents. However, the 2016 Baler dataset only had a two-year time resolution and a crude age model based on growth band counting. Here we present a new 2020 Baler I-129/I-127 atomic ratio dataset that features at least annual time resolution and a more accurate age model constructed using 3D X-ray Computed Tomography. Results show that the bomb peaks in Baler primarily came from the Pacific Proving Grounds or PPG with a time lag of about 1.8 years (or more specifically, between 1.3 and 2.4 years). Moreover, a review of the Pamla dataset shows that PPG signals may have been transported to Parola in the West Philippine Sea via two pathways: the northward and southward bifurcations of the North Equatorial Current, reaching Parola about 4.5 and 8.5 years after detonation, respectively. Moreover, a prominent peak in the year 2014.7 in Baler possibly came from the 2011 Fukushima Accident, transported by the Kuroshio Recirculation Gyre and the North Pacific Mode Waters with a 3.5-year time lag. This study contributes to the understanding of the impact and transport of human-made radionuclides to the Philippines and the relevant oceanographic processes in the Western Equatorial Pacific region.
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页数:9
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