Efficient organic light-emitting diodes fabricated on cellulose nanocrystal substrates

被引:39
作者
Najafabadi, E. [1 ]
Zhou, Y. H. [1 ]
Knauer, K. A. [1 ]
Fuentes-Hernandez, C. [1 ]
Kippelen, B. [1 ]
机构
[1] Georgia Inst Technol, Sch Elect & Comp Engn, COPE, Atlanta, GA 30332 USA
关键词
TRANSPARENT; NANOCOMPOSITE;
D O I
10.1063/1.4891046
中图分类号
O59 [应用物理学];
学科分类号
摘要
Organic light-emitting diodes (OLEDs) fabricated on recyclable and biodegradable substrates are a step towards the realization of a sustainable OLED technology. We report on efficient OLEDs with an inverted top-emitting architecture on recyclable cellulose nanocrystal (CNC) substrates. The OLEDs have a bottom cathode of Al/LiF deposited on a 400 nm thick N, N'-Di-[(1-naphthyl)-N, N'-diphenyl]-(1,1'-biphenyl)-4,4'-diamine (alpha-NPD) layer and a top anode of Au/MoO3. They achieve a maximum luminance of 74 591 cd/m(2) with a current efficacy of 53.7 cd/A at a luminance of 100 cd/m(2) and 41.7 cd/A at 1000 cd/m(2). It is shown that the alpha-NPD layer on the CNC substrate is necessary for achieving high performance OLEDs. The electroluminescent spectra of the OLEDs as a function of viewing angle are presented and show that the OLED spectra are subject to microcavity effects. (c) 2014 AIP Publishing LLC.
引用
收藏
页数:4
相关论文
共 28 条
[1]   Effect of reaction conditions on the properties and behavior of wood cellulose nanocrystal suspensions [J].
Beck-Candanedo, S ;
Roman, M ;
Gray, DG .
BIOMACROMOLECULES, 2005, 6 (02) :1048-1054
[2]   An effective cathode structure for inverted top-emitting organic light-emitting devices [J].
Chen, CW ;
Lin, CL ;
Wu, CC .
APPLIED PHYSICS LETTERS, 2004, 85 (13) :2469-2471
[3]   Inverted hybrid organic light-emitting device with polyethylene dioxythiophene-polystyrene sulfonate as an anode buffer layer [J].
Dobbertin, T ;
Werner, O ;
Meyer, J ;
Kammoun, A ;
Schneider, D ;
Riedl, T ;
Becker, E ;
Johannes, HH ;
Kowalsky, W .
APPLIED PHYSICS LETTERS, 2003, 83 (24) :5071-5073
[4]   Inverted top-emitting organic light-emitting diodes using sputter-deposited anodes [J].
Dobbertin, T ;
Kroeger, M ;
Heithecker, D ;
Schneider, D ;
Metzdorf, D ;
Neuner, H ;
Becker, E ;
Johannes, HH ;
Kowalsky, W .
APPLIED PHYSICS LETTERS, 2003, 82 (02) :284-286
[5]   Transparent and High Gas Barrier Films of Cellulose Nanofibers Prepared by TEMPO-Mediated Oxidation [J].
Fukuzumi, Hayaka ;
Saito, Tsuguyuki ;
Wata, Tadahisa ;
Kumamoto, Yoshiaki ;
Isogai, Akira .
BIOMACROMOLECULES, 2009, 10 (01) :162-165
[6]   Cellulose Nanocrystals: Chemistry, Self-Assembly, and Applications [J].
Habibi, Youssef ;
Lucia, Lucian A. ;
Rojas, Orlando J. .
CHEMICAL REVIEWS, 2010, 110 (06) :3479-3500
[7]   Chlorinated Indium Tin Oxide Electrodes with High Work Function for Organic Device Compatibility [J].
Helander, M. G. ;
Wang, Z. B. ;
Qiu, J. ;
Greiner, M. T. ;
Puzzo, D. P. ;
Liu, Z. W. ;
Lu, Z. H. .
SCIENCE, 2011, 332 (6032) :944-947
[8]   Top-emitting organic light-emitting diodes: Influence of cavity design [J].
Hofmann, Simone ;
Thomschke, Michael ;
Freitag, Patricia ;
Furno, Mauro ;
Luessem, Bjoern ;
Leo, Karl .
APPLIED PHYSICS LETTERS, 2010, 97 (25)
[9]   Transparent and conductive paper from nanocellulose fibers [J].
Hu, Liangbing ;
Zheng, Guangyuan ;
Yao, Jie ;
Liu, Nian ;
Weil, Ben ;
Eskilsson, Martin ;
Karabulut, Erdem ;
Ruan, Zhichao ;
Fan, Shanhui ;
Bloking, Jason T. ;
McGehee, Michael D. ;
Wagberg, Lars ;
Cui, Yi .
ENERGY & ENVIRONMENTAL SCIENCE, 2013, 6 (02) :513-518
[10]   Electroluminescence emission pattern of organic light-emitting diodes: Implications for device efficiency calculations [J].
Kim, JS ;
Ho, PKH ;
Greenham, NC ;
Friend, RH .
JOURNAL OF APPLIED PHYSICS, 2000, 88 (02) :1073-1081