CO2 reforming of CH4 by atmospheric pressure abnormal glow plasma

被引:0
|
作者
Chen, Qi [1 ]
Dai, Wei [1 ]
Tao, Xumei [1 ]
Yu, Hui [1 ]
Dai, Xiaoyan [1 ]
Yin, Yongxiang [1 ]
机构
[1] Sichuan Univ, Sch Chem Engn, Chengdu 610065, Peoples R China
关键词
abnormal glow plasma; methane; carbon dioxide; synthesis gas;
D O I
暂无
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
A novel plasma atmospheric pressure abnormal glow discharge was used to investigate synthesis gas production from reforming methane and carbon dioxide. Special attentions were paid to the discharge characteristics and CH4, CO2 conversion, H-2, CO selectivity, and ratio of H-2/CO varied with the changing of discharging power, the total flux, and the ratio of CH4/CO2. Experiments were performed in wider operation variables, the discharging power of 240 to 600 W, the CH4/CO2 of 0.2 to 1.0 and the total flux of 140 to 500 mL/min. The experiments showed that the conversion of CH4 and CO2 was up to 91.9% and 83.2%, the selectivity of CO and H-2 was also up to 80% and 90% and H-2/CO mole ratio was 0.2 to 1.2, respectively. A brief analysis for discharge characteristics and the experimental results were given.
引用
收藏
页码:181 / 184
页数:4
相关论文
共 50 条
  • [21] CH4-CO2 REFORMING IN THE PLASMA OF A NON-SELF-SUSTAINED DC GLOW DISCHARGE AT ATMOSPHERIC PRESSURE
    Arkhipenko, V., I
    Kazak, A., V
    Kirillov, A. A.
    Simonchik, L., V
    Tomkavich, M. U.
    HIGH TEMPERATURE MATERIAL PROCESSES, 2022, 26 (04): : 17 - 23
  • [22] Study on the conversion of CH4 and CO2 using a pulsed microwave plasma under atmospheric pressure
    Zhang, JQ
    Yang, YJ
    Zhang, JS
    Liu, Q
    ACTA CHIMICA SINICA, 2002, 60 (11) : 1973 - 1980
  • [23] Analysis of helium addition for enhancement of reactivity between CH4 and CO2 in atmospheric pressure plasma
    Duc Ba Nguyen
    Lee, Won Gyu
    JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY, 2015, 32 : 187 - 194
  • [24] Effects of pressure on CO2 reforming of CH4 over Rh catalysts.
    Srimat, ST
    Song, CS
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2000, 219 : U253 - U253
  • [25] Dry Reforming of CH4 With CO2 to Generate Syngas by Combined Plasma Catalysis
    Pan, Kuan Lun
    Chung, Wei Chieh
    Chang, Moo Been
    IEEE TRANSACTIONS ON PLASMA SCIENCE, 2014, 42 (12) : 3809 - 3818
  • [26] Effect of Different Feeding Modes on CO2 Reforming of CH4 by Thermal Plasma
    Bai Mei-Gui
    Tao Xu-Mei
    Wu Qing-You
    Huang Zhi-Jun
    Li Yu-Liang
    Yin Yong-Xiang
    Dai Xiao-Yan
    ACTA PHYSICO-CHIMICA SINICA, 2009, 25 (12) : 2455 - 2460
  • [27] CO2 Reforming of CH4 via Cold Plasma Jet Combined with Catalyst
    Yang Yungui
    Shang Shuyong
    Lin Na
    Yin Yongxiang
    Dai Xiaoyan
    APPLICATION OF CHEMICAL ENGINEERING, PTS 1-3, 2011, 236-238 : 596 - +
  • [28] A detailed mechanism of thermal CO2 reforming of CH4
    Wang, SG
    Li, YW
    Lu, JX
    He, MY
    Jiao, HJ
    JOURNAL OF MOLECULAR STRUCTURE-THEOCHEM, 2004, 673 (1-3): : 181 - 189
  • [29] Experiments for the reforming of CH4 with CO2 at high temperature
    Wang, Fang
    Gui, Keting
    Dongnan Daxue Xuebao (Ziran Kexue Ban)/Journal of Southeast University (Natural Science Edition), 2008, 38 (01): : 106 - 109
  • [30] Numerical investigation on the CH4/CO2 nanosecond pulsed dielectric barrier discharge plasma at atmospheric pressure
    Bai, Chengjie
    Wang, Lijuan
    Li, Li
    Dong, Xin
    Xiao, Qinghua
    Liu, Zhaoqian
    Sun, Jianhui
    Pan, Jie
    AIP ADVANCES, 2019, 9 (03)