Contribution of ZnO to Charge-Transfer Induced Surface-Enhanced Raman Scattering in Au/ZnO/PATP Assembly

被引:65
作者
Yang, Libin [1 ,2 ]
Ruan, Weidong [1 ]
Jiang, Xin [2 ]
Zhao, Bing [1 ]
Xu, Weiqing [1 ]
Lombardi, John R. [3 ]
机构
[1] Jilin Univ, State Key Lab Supramol Struct & Mat, Changchun 130012, Peoples R China
[2] Jiamusi Univ, Coll Chem & Pharmacol, Jiamusi 154007, Peoples R China
[3] CUNY City Coll, Dept Chem, New York, NY 10031 USA
基金
美国国家科学基金会;
关键词
RESOLVED NANOSPHERE LITHOGRAPHY; FERMI-LEVEL EQUILIBRATION; SILVER ELECTRODE; OPTICAL-PROPERTIES; P-AMINOTHIOPHENOL; SPECTROSCOPY; SERS; NANOPARTICLES; MOLECULES; PYRIDINE;
D O I
10.1021/jp8074095
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The assembly of metal/semiconductor/molecule was fabricated with gold nanoparticles, ZnO, and 4-aminothiophenol (PATP) molecules through the layer-by-layer self-assembly method. Raman spectra of PATP adsorbed on Au/ZnO were considerably enhanced relative to those observed on Au particles alone. By examining the relative enhancement of the nontotally symmetric (b(2)) modes, this effect is shown to arise from a charge transfer (CT) contribution from the metal to molecule.
引用
收藏
页码:117 / 120
页数:4
相关论文
共 35 条
[21]   SURFACE SELECTION-RULES FOR SURFACE-ENHANCED RAMAN-SPECTROSCOPY - CALCULATIONS AND APPLICATION TO THE SURFACE-ENHANCED RAMAN-SPECTRUM OF PHTHALAZINE ON SILVER [J].
MOSKOVITS, M ;
SUH, JS .
JOURNAL OF PHYSICAL CHEMISTRY, 1984, 88 (23) :5526-5530
[22]   SURFACE-ENHANCED SPECTROSCOPY [J].
MOSKOVITS, M .
REVIEWS OF MODERN PHYSICS, 1985, 57 (03) :783-826
[23]   CHARGE-TRANSFER RESONANCE RAMAN PROCESS IN SURFACE-ENHANCED RAMAN-SCATTERING FROM P-AMINOTHIOPHENOL ADSORBED ON SILVER - HERZBERG-TELLER CONTRIBUTION [J].
OSAWA, M ;
MATSUDA, N ;
YOSHII, K ;
UCHIDA, I .
JOURNAL OF PHYSICAL CHEMISTRY, 1994, 98 (48) :12702-12707
[24]   SURFACE-ENHANCED RAMAN-SCATTERING [J].
OTTO, A ;
MROZEK, I ;
GRABHORN, H ;
AKEMANN, W .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1992, 4 (05) :1143-1212
[25]   Observation of molecules adsorbed on III-V semiconductor quantum dots by surface-enhanced Raman scattering [J].
Quagliano, LG .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2004, 126 (23) :7393-7398
[26]   Optical properties of two interacting gold nanoparticles [J].
Rechberger, W ;
Hohenau, A ;
Leitner, A ;
Krenn, JR ;
Lamprecht, B ;
Aussenegg, FR .
OPTICS COMMUNICATIONS, 2003, 220 (1-3) :137-141
[27]   Surface-enhanced Raman scattering in the ultraviolet spectral region: UV-SERS on rhodium and ruthenium electrodes [J].
Ren, B ;
Lin, XF ;
Yang, ZL ;
Liu, GK ;
Aroca, RF ;
Mao, BW ;
Tian, ZQ .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2003, 125 (32) :9598-9599
[28]   Green emission to probe photoinduced charging events in ZnO-Au nanoparticles. Charge distribution and fermi-level equilibration [J].
Subramanian, V ;
Wolf, EE ;
Kamat, PV .
JOURNAL OF PHYSICAL CHEMISTRY B, 2003, 107 (30) :7479-7485
[29]   Expanding generality of surface-enhanced Raman spectroscopy with borrowing SERS activity strategy [J].
Tian, Zhong-Qun ;
Ren, Bin ;
Li, Jian-Feng ;
Yang, Zhi-Lin .
CHEMICAL COMMUNICATIONS, 2007, (34) :3514-3534
[30]   Surface-enhanced Raman scattering: From noble to transition metals and from rough surfaces to ordered nanostructures [J].
Tian, ZQ ;
Ren, B ;
Wu, DY .
JOURNAL OF PHYSICAL CHEMISTRY B, 2002, 106 (37) :9463-9483