Piezoelectric potential induced the improved micro-pollutant dye degradation of Co doped MoS2 ultrathin nanosheets in dark

被引:54
作者
Yein, Win Thi [1 ]
Wang, Qun [1 ]
Li, Yang [1 ]
Wu, Xiaohong [1 ]
机构
[1] Harbin Inst Technol, Sch Chem & Chem Engn, MIIT Key Lab Crit Mat Technol New Energy Convers, Harbin 150001, Heilongjiang, Peoples R China
基金
中国国家自然科学基金;
关键词
Doping; MoS2; Piezocatalytic; Degradation; Organic dye; PHOTOCATALYSIS; NANOWIRES; CATALYSIS; ENERGY;
D O I
10.1016/j.catcom.2019.03.023
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The few number layers of Co doped MoS2 ultrathin nanosheets (UNs) with the thickness of 3.2 nm were successfully fabricated, which can decompose MB dye by 99% in 60 s through ultrasonic wave vibration in dark. Co doped MoS2 UNs (Co-MoS2-0.10) exhibited the higher piezoelectric catalytic performance than that of its counterparts. Moreover, to verify the enhanced piezoelectric catalytic activity of MoS2 via doping effect, molecular oxygen activation properties are monitored by superoxide radical (O-center dot(2)-) and hydroxyl radical ((OH)-O-center dot) evolution. In addition, the piezoelectric degradation mechanism of pollutant dye had also been investigated in detail.
引用
收藏
页码:61 / 65
页数:5
相关论文
共 23 条
[1]   Facet-Engineered Surface and Interface Design of Photocatalytic Materials [J].
Bai, Song ;
Wang, Lili ;
Li, Zhengquan ;
Xiong, Yujie .
ADVANCED SCIENCE, 2017, 4 (01)
[2]   Curved surface TiO2 nanodrums coupled with MoS2 as heterojunction photocatalysts with enhancing photocatalytic activity [J].
Chen, Xuan ;
Zhang, Jun ;
Jiang, Xudong ;
Wang, Hongbo ;
Kong, Zhe ;
Xi, Junhua ;
Ji, Zhenguo .
MATERIALS LETTERS, 2018, 229 :277-280
[3]   Multiscale structural and electronic control of molybdenum disulfide foam for highly efficient hydrogen production [J].
Deng, Jiao ;
Li, Haobo ;
Wang, Suheng ;
Ding, Ding ;
Chen, Mingshu ;
Liu, Chuan ;
Tian, Zhongqun ;
Novoselov, K. S. ;
Ma, Chao ;
Deng, Dehui ;
Bao, Xinhe .
NATURE COMMUNICATIONS, 2017, 8
[4]   Multifunctional Bi2O2(OH)(NO3) Nanosheets with {001} Active Exposing Facets: Efficient Photocatalysis, Dye-Sensitization, and Piezoelectric-Catalysis [J].
Hao, Lin ;
Huang, Hongwei ;
Guo, Yuxi ;
Zhang, Yihe .
ACS SUSTAINABLE CHEMISTRY & ENGINEERING, 2018, 6 (02) :1848-1862
[5]   High Piezo-photocatalytic Efficiency of CuS/ZnO Nanowires Using Both Solar and Mechanical Energy for Degrading Organic Dye [J].
Hong, Deyi ;
Zang, Weili ;
Guo, Xiao ;
Fu, Yongming ;
He, Haoxuan ;
Sun, Jing ;
Xing, Lili ;
Liu, Baodan ;
Xue, Xinyu .
ACS APPLIED MATERIALS & INTERFACES, 2016, 8 (33) :21302-21314
[6]   Macroscopic Polarization Enhancement Promoting Photo- and Piezoelectric-Induced Charge Separation and Molecular Oxygen Activation [J].
Huang, Hongwei ;
Tu, Shuchen ;
Zeng, Chao ;
Zhang, Tierui ;
Reshak, Ali H. ;
Zhang, Yihe .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2017, 56 (39) :11860-11864
[7]   State-of-the-Art Progress in Diverse Heterostructured Photocatalysts toward Promoting Photocatalytic Performance [J].
Li, Haijin ;
Zhou, Yong ;
Tu, Wenguang ;
Ye, Jinhua ;
Zou, Zhigang .
ADVANCED FUNCTIONAL MATERIALS, 2015, 25 (07) :998-1013
[8]   Cobalt-Doping in Molybdenum-Carbide Nanowires Toward Efficient Electrocatalytic Hydrogen Evolution [J].
Lin, Huanlei ;
Liu, Ning ;
Shi, Zhangping ;
Guo, Yulin ;
Tang, Yi ;
Gao, Qingsheng .
ADVANCED FUNCTIONAL MATERIALS, 2016, 26 (31) :5590-5598
[9]   Single- and few-layers MoS2 nanocomposite as piezo-catalyst in dark and self-powered active sensor [J].
Lin, Jyun-Hao ;
Tsao, Yu-Hsiang ;
Wu, Mei-Hsuan ;
Chou, Ting-Mao ;
Lin, Zong-Hong ;
Wu, Jyh Ming .
NANO ENERGY, 2017, 31 :575-581
[10]  
Liu W., 2018, NANO ENERGY, V44, P111, DOI [10.1016/j.nanoen.2017.11.010, DOI 10.1016/J.NANOEN.2017.11.010, DOI 10.1016/J.NANOEN.2017.12.034]