Review: mechanisms and consequences of chemical cross-talk in advanced Li-ion batteries

被引：78

作者：

Harris, Oliver C. ^{[1
]}

Lee, Sophia E. ^{[1
]}

Lees, Cassandra ^{[1
]}

Tang, Maureen ^{[1
]}

机构：

[1] Drexel Univ, Dept Chem & Biol Engn, Philadelphia, PA 19104 USA

来源：

JOURNAL OF PHYSICS-ENERGY | 2020年 / 2卷 / 03期

关键词：

electrode cross-talk; capacity fade; battery lifetime; SELF-DISCHARGE MECHANISM; LITHIUM-ION; ELECTROCHEMICAL REDUCTION; SINGLET OXYGEN; METAL DISSOLUTION; OXIDATION-STATE; CARBON-DIOXIDE; SIDE-REACTIONS; CAPACITY FADE; REDOX SHUTTLE;

D O I：

10.1088/2515-7655/ab8b68

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Electrode cross-talk in Li-ion batteries refers to side reactions in which soluble products are generated at one electrode and consumed or further reacted at the other electrode. While these reactions impact battery lifetime directly, they perhaps have even greater consequence for battery management systems and state-of-health prediction. In this work, we review the current literature on cross-talk mechanisms, classify various reactions as firmly detrimental or beneficial to cell lifetime, and identify future scientific challenges in the area.

引用

页数：21

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