Possible change in Asian dust source suggested by atmospheric anthropogenic radionuclides during the 2000s

Decades-long monitoring of anthropogenic radionuclides in the atmospheric deposition in Tsukuba, Japan suggests not only the substantial impacts of the Asian dust (Kosa) on the deposition but also the possible change of the Kosa source region, especially during springs of the 2000s. In order to know more about such change, 4 single wet deposition events occurred in the spring of 2007 were scrutinized. The largest anthropogenic radionuclides wet deposition was supplied by the April 2-4 event. It brought several tens % of the monthly depositions (April 2007) of the dust (residue) mass (4.5 g m(-2)) and anthropogenic radionulides (Sr-90: 16, Cs-137: 97 and Pu: 3 mBq m(-2)). None of the events observed fulfilled both criteria of the specific activities and Sr-90/Cs-137 activity ratio to the Tsukuba soil; they did not exhibit local soil dust signature. The Kosa events in fact have extensive impacts on the atmospheric environment over Japan in spring season. Considering the elevated specific activities as well as greater Cs-137/Sr-90 activity ratio in the deposited dust, it is hypothesized that the dust source areas in Asian continent would be shifting from the and zone to the desert-steppe zone suffering from desertification during the 2000s. This type of the Kosa may be called as the 'new-regime Kosa'. Chemical observation in the far downwind region of the Kosa dust could allow us to know possible shift in the source regions. (C) 2009 Elsevier Ltd. All rights reserved.