Visible-Light-Driven BiOI-Based Janus Micromotor in Pure Water

被引:317
作者
Dong, Renfeng [1 ]
Hu, Yan [2 ]
Wu, Yefei [2 ]
Gao, Wei [3 ,4 ]
Ren, Biye [2 ]
Wang, Qinglong [1 ]
Cai, Yuepeng [1 ]
机构
[1] South China Normal Univ, Guangdong Prov Engn Technol Res Ctr Mat Energy Co, Guangzhou Key Lab Mat Energy Convers & Storage, Sch Chem & Environm, Guangzhou 510006, Guangdong, Peoples R China
[2] South China Univ Technol, Sch Mat Sci & Engn, Guangzhou 510640, Guangdong, Peoples R China
[3] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA
[4] Univ Calif Berkeley, Berkeley Sensor & Actuator Ctr, Berkeley, CA 94720 USA
基金
中国博士后科学基金;
关键词
BIOMEDICAL APPLICATIONS; CATALYTIC NANOMOTORS; TUBULAR MICROENGINES; AUTONOMOUS MOVEMENT; MOTORS; IRRADIATION; PROPULSION; BR; MICRO/NANOMOTORS; PHOTOCATALYSTS;
D O I
10.1021/jacs.6b09863
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Light-driven synthetic micro-/nanomotors have attracted considerable attention due to their potential applications and unique performances such as remote motion control and adjustable velocity. Utilizing harmless and renewable visible light to supply energy for micro-/nanomotors in water represents a great challenge. In view of the outstanding photocatalytic performance of bismuth oxyiodide visible-light-driven BiOI-based Janus micromotors have been developed, which can be activated by a broad spectrum of light, including blue and green light. Such BiOI-based Janus micromotors can be propelled by photocatalytic reactions in pure water under environmentally friendly visible light without the addition of any other chemical fuels. The remote control of photocatalytic propulsion by modulating the power of visible light is characterized by velocity and mean-square displacement analysis of optical video recordings. In addition, the self-electrophoresis mechanism has been confirmed for such visible-light-driven BiOI-based Janus micromotors by demonstrating the effects of various coated layers (e.g., Al2O3, Pt, and Au) on the velocity of motors. The successful demonstration of visible-light driven Janus micromotors holds a great promise for future biomedical and environmental applications.
引用
收藏
页码:1722 / 1725
页数:4
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