Influence of mineralization and injection flow rate on flow patterns in three-dimensional porous media

被引:11
作者
Moosavi, R. [1 ]
Kumar, A. [1 ]
De Wit, A. [2 ]
Schroeter, M. [1 ]
机构
[1] MPIDS, D-37077 Gottingen, Germany
[2] ULB, Nonlinear Phys Chem Unit, CP231, B-1050 Brussels, Belgium
关键词
PORE-SCALE; MULTIPHASE FLOW; REACTIVE FLOW; DISSOLUTION; PRECIPITATION; LIMESTONE; PERMEABILITY; EVOLUTION; POROSITY; HETEROGENEITY;
D O I
10.1039/c9cp01382b
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Reactive flows inside porous media play an important role in a number of geophysical and industrial processes. Here, we present three-dimensional experimental measurements on how precipitation and flow patterns change with the flow rate inside a model porous medium consisting of monodisperse glass beads. The sample is initially filled with an aqueous solution of sodium carbonate into which a solution of barium chloride is injected at a constant flow rate. Upon contact and reaction, the two reactants produce water-insoluble barium carbonate which precipitates onto the glass beads. This precipitate then modifies the flow morphology which in turn changes the spatial distribution of the precipitate. We discuss the influence of the flow rate on the morphology of the flow pattern and demonstrate that neither viscous fingering nor the Rayleigh-Taylor instability have any significant influence in our model system.
引用
收藏
页码:14605 / 14611
页数:7
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