Extending FRET cascades on linear DNA photonic wires

被引:59
作者
Spillmann, Christopher M. [1 ]
Buckhout-White, Susan [1 ,2 ]
Oh, Eunkeu [3 ,4 ]
Goldman, Ellen R. [1 ]
Ancona, Mario G. [3 ]
Medintz, Igor L. [1 ]
机构
[1] US Naval Res Lab, Ctr Bio Mol Sci & Engn, Washington, DC 20375 USA
[2] George Mason Univ, Coll Sci, Fairfax, VA 22030 USA
[3] US Naval Res Lab, Elect Sci & Technol Div, Div Opt Sci, Washington, DC 20375 USA
[4] Sotera Def Solut, Columbia, MD 21046 USA
关键词
RESONANCE ENERGY-TRANSFER; 3-WAY JUNCTION; NANOTECHNOLOGY; SYSTEMS;
D O I
10.1039/c4cc01072h
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Photonic wires were constructed by sequentially arranging up to 7 fluorophores along a concatenated DNA scaffold. This yielded nanostructures displaying from one- to six-energy transfer steps where end-to-end efficiency reflected the multiple underlying photophysical processes and the ability of long-range interactions to compensate for localized non-ideal dye behaviour.
引用
收藏
页码:7246 / 7249
页数:4
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