Highly Efficient and Recyclable Carbon Soot Sponge for Oil Cleanup

被引:152
作者
Gao, Yang [1 ]
Zhou, Yun Shen [1 ]
Xiong, Wei [1 ]
Wang, Mengmeng [2 ]
Fan, Lisha [1 ]
Rabiee-Golgir, Hossein [1 ]
Jiang, Lijia [1 ]
Hou, Wenjia [1 ]
Huang, Xi [1 ]
Jiang, Lan [2 ]
Silvain, Jean-Francois [3 ]
Lu, Yong Feng [1 ]
机构
[1] Univ Nebraska, Dept Elect Engn, Lincoln, NE 68588 USA
[2] Beijing Inst Technol, Sch Mech Engn, Laser Micro Nano Fabricat Lab, Beijing 10008, Peoples R China
[3] Univ Bordeaux 1, CNRS, ICMCB, F-33608 Pessac, France
基金
美国国家科学基金会;
关键词
carbon soot sponge; hydrophobicity; water contact angle; oil absorption; environment protection; CANDLE SOOT; GRAPHENE; FOAM; ABSORPTION; NANOTUBES; ROBUST; SEPARATION; MEMBRANES; SORPTION; WATER;
D O I
10.1021/am500870f
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Carbon soot (CS) has the advantages of cost-effectiveness and production scalability over other carbons (i.e., graphene, CNTs) in their synthesis. However, little research has been conducted to explore the potential applications of CS. In this study, we demonstrated that a.common daily waste-CS-can be used for developing a cost-effective absorbent (CS-sponge) to remove oil contaminants from water. The CS was synthesized by an ethylene-oxygen combustion flame. The CS-sponge was prepared via a dip-coating method. Without further surface modification and pretreatments, the CS-sponge demonstrates high absorption capacities (up to 80 times its own weight) for a broad spectrum of oils and organic solvents with a recyclability of more than 10 times. These research results show evidence that the CS-sponge is promising in environmental remediation for large-scale, low-cost removal of oils from water.
引用
收藏
页码:5924 / 5929
页数:6
相关论文
共 37 条
[1]   Engines and exhaust after treatment systems for future automotive applications [J].
Alkemade, Ulrich G. ;
Schumann, Bemd .
SOLID STATE IONICS, 2006, 177 (26-32) :2291-2296
[2]   MOF derived porous carbon-Fe3O4 nanocomposite as a high performance, recyclable environmental superadsorbent [J].
Banerjee, Abhik ;
Gokhale, Rohan ;
Bhatnagar, Sumit ;
Jog, Jyoti ;
Bhardwaj, Monika ;
Lefez, Benoit ;
Hannoyer, Beatrice ;
Ogale, Satishchandra .
JOURNAL OF MATERIALS CHEMISTRY, 2012, 22 (37) :19694-19699
[3]   Spongy Graphene as a Highly Efficient and Recyclable Sorbent for Oils and Organic Solvents [J].
Bi, Hengchang ;
Xie, Xiao ;
Yin, Kuibo ;
Zhou, Yilong ;
Wan, Shu ;
He, Longbing ;
Xu, Feng ;
Banhart, Florian ;
Sun, Litao ;
Ruoff, Rodney S. .
ADVANCED FUNCTIONAL MATERIALS, 2012, 22 (21) :4421-4425
[4]   Effects of firing coal and biomass under oxy-fuel conditions in a power plant boiler using CFD modelling [J].
Black, S. ;
Szuhanszki, J. ;
Pranzitelli, A. ;
Ma, L. ;
Stanger, P. J. ;
Ingham, D. B. ;
Pourkashanian, M. .
FUEL, 2013, 113 :780-786
[5]   Elastic carbon foam via direct carbonization of polymer foam for flexible electrodes and organic chemical absorption [J].
Chen, Shuiliang ;
He, Guanghua ;
Hu, Huan ;
Jin, Shaoqin ;
Zhou, Yan ;
He, Yunyun ;
He, Shuijian ;
Zhao, Feng ;
Hou, Haoqing .
ENERGY & ENVIRONMENTAL SCIENCE, 2013, 6 (08) :2435-2439
[6]   Chemical and morphological characteristics of indoor and outdoor particulate matter in an urban environment [J].
Chithra, V. S. ;
Nagendra, S. M. Shiva .
ATMOSPHERIC ENVIRONMENT, 2013, 77 :579-587
[7]   A Polydimethylsiloxane (PDMS) Sponge for the Selective Absorption of Oil from Water [J].
Choi, Sung-Jin ;
Kwon, Tae-Hong ;
Im, Hwon ;
Moon, Dong-Il ;
Baek, David J. ;
Seol, Myeong-Lok ;
Duarte, Juan P. ;
Choi, Yang-Kyu .
ACS APPLIED MATERIALS & INTERFACES, 2011, 3 (12) :4552-4556
[8]   Three-Dimensionally Macroporous Fe/C Nanocomposites As Highly Selective Oil-Absorption Materials [J].
Chu, Ying ;
Pan, Qinmin .
ACS APPLIED MATERIALS & INTERFACES, 2012, 4 (05) :2420-2425
[9]   Macroscopic Multifunctional Graphene-Based Hydrogels and Aerogels by a Metal Ion Induced Self-Assembly Process [J].
Cong, Huai-Ping ;
Ren, Xiao-Chen ;
Wang, Ping ;
Yu, Shu-Hong .
ACS NANO, 2012, 6 (03) :2693-2703
[10]   Candle Soot as a Template for a Transparent Robust Superamphiphobic Coating [J].
Deng, Xu ;
Mammen, Lena ;
Butt, Hans-Juergen ;
Vollmer, Doris .
SCIENCE, 2012, 335 (6064) :67-70