5-Hydroxymethylfurfural Production from Glucose, Fructose, Cellulose, or Cellulose-based Waste Material by Using a Calcium Phosphate Catalyst and Water as a Green Solvent

被引：22
|
作者：
Mimura, Naoki [1 ]
Sato, Osamu [1 ]
Shirai, Masayuki [1 ,2 ]
Yamaguchi, Aritomo [1 ,3 ]
机构：
[1] Natl Inst Adv Ind Sci & Technol, Res Inst Chem Proc Technol, Miyagino Ku, 4-2-1 Nigatake, Sendai, Miyagi 9838551, Japan
[2] Iwate Univ, Dept Chem & Bioengn, Fac Engn, Ueda 4-3-5, Morioka, Iwate 0208551, Japan
[3] JST, PRESTO, Miyagino Ku, 4-2-1 Nigatake, Sendai, Miyagi 9838551, Japan
来源：
CHEMISTRYSELECT | 2017年 / 2卷 / 03期
基金：
日本学术振兴会;
关键词：
Biomass; Green chemistry; Heterogeneous catalysis; 5-Hydroxymethylfurfural; Water solvent; HYDROXYAPATITE CATALYSTS; AEROBIC OXIDATION; SELECTIVE HYDROGENATION; LIGNOCELLULOSIC BIOMASS; ACID; CONVERSION; DEHYDRATION; CARBON; HMF; 2,5-DIFORMYLFURAN;
D O I：
10.1002/slct.201601869
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
We successfully prepared 5-hydroxymethylfurfural from glucose, fructose, cellulose, natural wood, waste paper, and cotton clothing by using a calcium phosphate catalyst and water as a green solvent. The combination of basic and acidic sites on the surface of the calcium phosphate catalyst accelerated the multistep reaction pathway from the reactants to 5-hydroxymethylfurfural. Ball-milling pretreatment of the reactant markedly increased the yield of 5-hydroxymethylfurfural obtained from cellulose, natural wood, waste paper, and cotton clothing.
引用
收藏
页码：1305 / 1310
页数：6
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