Experimental measurements of short-lived fission products from uranium, neptunium, plutonium and americium

被引:13
作者
Metz, Lori A. [1 ]
Payne, Rosara F. [1 ]
Friese, Judah I. [1 ]
Greenwood, Larry R. [1 ]
Kephart, Jeremy D. [1 ]
Pierson, Bruce D. [1 ]
机构
[1] Pacific NW Natl Lab, Richland, WA 99352 USA
关键词
Fission products; Short-lived radionuclides; Research reactor experiments; Actinide fission; GAMMA-RAYS; ENERGY;
D O I
10.1007/s10967-009-0225-1
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
Fission yields are especially well characterized for long-lived fission products. Modeling techniques incorporate numerous assumptions and can be used to deduce information about the distribution of short-lived fission products. This work is an attempt to gather experimental (model-independent) data on short-lived fission products. Fissile isotopes of uranium, neptunium, plutonium and americium were irradiated under pulse conditions at the Washington State University 1 MW TRIGA reactor to achieve similar to 10(8) fissions. The samples were placed on an HPGe (high purity germanium) detector to initiate counting in less than 3 min post irradiation. The data was analyzed to determine which radionuclides could be quantified and compared to the published fission yield data.
引用
收藏
页码:373 / 377
页数:5
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