Modeling fractal aggregates of polydisperse particles with tunable dimension

被引:21
作者
Tomchuk, Oleksandr, V [1 ,2 ]
Avdeev, Mikhail, V [1 ,3 ]
Bulavin, Leonid A. [2 ]
机构
[1] Joint Inst Nucl Res, Frank Lab Neutron Phys, Dubna 141980, Moscow Region, Russia
[2] Taras Shevchenko Natl Univ Kyiv, Fac Phys, UA-03022 Kiev, Ukraine
[3] Dubna State Univ, Dubna 141982, Moscow Region, Russia
关键词
Fractal; Aggregate numerical generation; Polydispersity; Small-angle scattering; SMALL-ANGLE SCATTERING; DIFFUSION-LIMITED AGGREGATION; CLUSTER-CLUSTER AGGREGATION; NEUTRON-SCATTERING; SIZE DISTRIBUTION; LIGHT-SCATTERING; SIMULATION; MORPHOLOGY; GEOMETRY; GROWTH;
D O I
10.1016/j.colsurfa.2020.125331
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A generalized non-kinetic off-lattice algorithm to construct stochastic fractal clusters of polydisperse particles with tunable cluster parameters including dimension, is presented. The model based on a hierarchical procedure extends the previous studies in this area to the general case of the cluster-cluster aggregation and, in contrast to the previous kinetic models, makes it possible to generate clusters with a continuous change in the structure, in particular, covering the full range of natural mass fractal dimensions between one and three. An example of the morphological study of numerically generated clusters based on the correlation analysis in both direct and reciprocal spaces is given. In the latter case, it is demonstrated that the use of the developed fast algorithm gives an accurate and self-consistent description of the small-angle scattering data.
引用
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页数:8
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