Removal of Tetracycline Hydrochloride from Water by Visible-Light Photocatalysis Using BiFeO3/BC Materials

被引:7
作者
Fang, Zhengyang [1 ,2 ]
Jiang, Honghui [1 ]
Gong, Jiamin [1 ]
Zhang, Hengrui [1 ]
Hu, Xi [1 ]
Ouyang, Ke [1 ]
Guo, Yuan [3 ]
Hu, Xinjiang [1 ]
Wang, Hui [1 ,4 ]
Wang, Ping [1 ]
机构
[1] Cent South Univ Forestry & Technol, Coll Environm Sci & Engn, Changsha 410004, Peoples R China
[2] Guangzhou Inst Geochem, Chinese Acad Sci, Guangzhou 510640, Peoples R China
[3] Inst Bast Fiber Crops, Chinese Acad Agr Sci, Changsha 410205, Peoples R China
[4] Cent South Univ Forestry & Technol, Fac Life Sci & Technol, Changsha 410004, Peoples R China
基金
中国国家自然科学基金;
关键词
tetracycline hydrochloride; pharmaceutical wastewater; biochar; photocatalysis; kinetics; visible light; AQUEOUS-SOLUTION; DEGRADATION; ADSORPTION; BIOCHAR; MECHANISM; ANTIBIOTICS; KINETICS;
D O I
10.3390/catal12111461
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
It is widely considered that photocatalysis is an effective and eco-friendly method of dealing with organic pollutants dissolved in water. Nonetheless, photocatalysts still have some drawbacks, such as poor visible-light absorption, easy recombination of photogenerated charge carriers, and limited active sites. In this study, bismuth ferrite coupled with biochar material (BiFeO3/BC) was simply synthesized, and its photocatalysis reactivity was systemically examined under an irradiation of lambda > 400 nm. The experimental results showed that under a relatively acidic environment, the removal rate of tetracycline hydrochloride reached 95%. Using a variety of characterization investigations, we analyzed the morphology structure and chemical composition of BiFeO3/BC. In consideration of simple preparation and high respondence toward visible light, further explorations of BiFeO3/BC and its properties and optimized degradation conditions are worthwhile.
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页数:12
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共 58 条
[1]   Size-dependent structural parameters, optical, and magnetic properties of facile synthesized pure-phase BiFeO3 [J].
Alikhanov, Nariman M-R ;
Rabadanov, Murtazali Kh ;
Orudzhev, Farid F. ;
Gadzhimagomedov, Sultanakhmed Kh ;
Emirov, Ruslan M. ;
Sadykov, Sadyk A. ;
Kallaev, Suleiman N. ;
Ramazanov, Shikhgasan M. ;
Abdulvakhidov, Kamaludin G. ;
Sobola, Dinara .
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2021, 32 (10) :13323-13335
[2]   Photocatalytic pathway toward degradation of environmental pharmaceutical pollutants: structure, kinetics and mechanism approach [J].
Bagheri, Samira ;
TermehYousefi, Amin ;
Do, Trong-On .
CATALYSIS SCIENCE & TECHNOLOGY, 2017, 7 (20) :4548-4569
[3]   Uncovering the systematical charge separation effect of boron nitride quantum dots on photocatalytic performance of BiFeO3 perovskite towards degradation of tetracycline antibiotic [J].
Balta, Zeynep ;
Simsek, Esra Bilgin .
JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, 2021, 9 (06)
[4]   Experimental Evidence for the Carrier Transportation Enhanced Visible Light Driven Photocatalytic Process in Bismuth Ferrite (BiFeO3) One-Dimensional Fiber Nanostructures [J].
Bharathkumar, S. ;
Sakar, M. ;
Balakumar, S. .
JOURNAL OF PHYSICAL CHEMISTRY C, 2016, 120 (33) :18811-18821
[5]   Removal of lead(II) from water using activated carbon developed from jujube stones, a low-cost sorbent [J].
Bouchelkia, Nasma ;
Mouni, Lotfi ;
Belkhiri, Lazhar ;
Bouzaza, Abdelkrim ;
Bollinger, Jean-Claude ;
Madani, Khoudir ;
Dahmoune, Farid .
SEPARATION SCIENCE AND TECHNOLOGY, 2016, 51 (10) :1645-1653
[6]   Design and Preparation of Chitosan-Crosslinked Bismuth Ferrite/Biochar Coupled Magnetic Material for Methylene Blue Removal [J].
Cai, Xiaoxi ;
Li, Jiang ;
Liu, Yunguo ;
Hu, Xinjiang ;
Tan, Xiaofei ;
Liu, Shaobo ;
Wang, Hui ;
Gu, Yanling ;
Luo, Lerong .
INTERNATIONAL JOURNAL OF ENVIRONMENTAL RESEARCH AND PUBLIC HEALTH, 2020, 17 (01)
[7]   Facile synthesis of Co(II)-BiOCl@biochar nanosheets for photocatalytic degradation of p-nitrophenol under vacuum ultraviolet (VUV) irradiation [J].
Cao, Ting-ting ;
Cui, Han ;
Zhang, Qi-wei ;
Cui, Chong-wei .
APPLIED SURFACE SCIENCE, 2021, 559
[8]   Visible-light photocatalytic properties of weak magnetic BiFeO3 nanoparticles [J].
Gao, Feng ;
Chen, Xinyi ;
Yin, Kuibo ;
Dong, Shuai ;
Ren, Zhifeng ;
Yuan, Fang ;
Yu, Tao ;
Zou, Zhigang ;
Liu, Jun-Ming .
ADVANCED MATERIALS, 2007, 19 (19) :2889-+
[9]   Cell wall modification induced by an arbuscular mycorrhizal fungus enhanced cadmium fixation in rice root [J].
Gao, Meng Ying ;
Chen, Xun Wen ;
Huang, Wei Xiong ;
Wu, Li ;
Yu, Zheng Sheng ;
Xiang, Lei ;
Mo, Ce Hui ;
Li, Yan Wen ;
Cai, Quan Ying ;
Wong, Ming Hung ;
Li, Hui .
JOURNAL OF HAZARDOUS MATERIALS, 2021, 416
[10]   Tetracyclines in Food and Feedingstuffs: From Regulation to Analytical Methods, Bacterial Resistance, and Environmental and Health Implications [J].
Granados-Chinchilla, Fabio ;
Rodriguez, Cesar .
JOURNAL OF ANALYTICAL METHODS IN CHEMISTRY, 2017, 2017