High-Temperature Investigation of TeO2-Na2O-ZnO Glasses

被引：3
作者：
de Clermont-Gallerande, Jonathan [1 ]
Taniguchi, Daiki [1 ]
Colas, Maggy [2 ]
Thomas, Philippe [2 ]
Hayakawa, Tomokatsu [1 ,3 ]
机构：
[1] Nagoya Inst Technol, Dept Life Sci & Appl Chem, Field Adv Ceram, Showa Ku, Nagoya, Aichi 4668555, Japan
[2] Univ Limoges, Inst Rech Ceram IRCER, UMR 7315, Ctr Europeen Ceram,CNRS, 12 Rue Atlantis, F-87068 Limoges, France
[3] Nagoya Inst Technol, Frontier Res Inst Mat Sci FRIMS, Showa Ku, Nagoya, Aichi 4668555, Japan
来源：
PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS | 2022年 / 259卷 / 09期
基金：
日本学术振兴会;
关键词：
high temperatures; Raman; tellurite; thermal evolution; X-ray diffraction; NONLINEAR-OPTICAL PROPERTIES; RAMAN-SPECTRA; STRUCTURAL-PROPERTIES; THERMAL-CHARACTERISTICS; TEO2-RICH PART; PHASES; SYSTEM;
D O I：
10.1002/pssb.202200065
中图分类号：
O469 [凝聚态物理学];
学科分类号：
070205 ;
摘要：
Herein, a ternary system of TeO2-ZnO-Na2O (TZN) with competitive roles of covalent Zn-O and ionic Na-O bonds in tellurite glassy network is examined for high-temperature in situ X-ray diffraction (XRD) and Raman spectroscopy. TZN glasses are doped with Nd2O3 and the effects of Nd doping on the crystallization of glasses are also written. In situ high-temperature XRD permits the assignment of each of the differential scanning calorimetry (DSC) crystallization peaks (the first crystallization peak (T-c(1)) is related to sodium-based crystalline phases, while the second crystallization peak (T-c(2)) is correlated with tellurium-/zinc-based crystalline phases). The study of in situ high-temperature Raman spectroscopy shows that T-c1 shows gamma-TeO2 crystallized phase-like peaks while T-c2 crystallization has more alpha-TeO2-crystallized phase-like peaks. Comparison at the same temperature (430 degrees C) permits a first understanding of the structural changes of the glasses in terms of the evolution first to alpha-TeO2, ZnO, ZnTeO3, and Zn(2)Te(3)O(8 )crystalline phases compared with Na10Zn4O9 phase. The ZnTeO3 and Zn2Te3O8 crystallization evolution is also compared between the Nd-doped and nondoped glasses, which gives more insight into the tellurite glass structures.
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页数：7
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