Exploring the Molecular Conformation Space by Soft Molecule- Surface Collision

被引:49
作者
Anggara, Kelvin [1 ]
Zhu, Yuntao [2 ]
Delbianco, Martina [2 ]
Rauschenbach, Stephan [1 ,3 ]
Abb, Sabine [1 ]
Seeberger, Peter H. [2 ,4 ]
Kern, Klaus [1 ,5 ]
机构
[1] Max Planck Inst Solid State Res, DE-70569 Stuttgart, Germany
[2] Max Planck Inst Colloids & Interfaces, DE-14476 Potsdam, Germany
[3] Univ Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England
[4] Free Univ Berlin, Dept Chem & Biochem, DE-14195 Berlin, Germany
[5] Inst Phys, Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland
关键词
X-RAY; AMORPHOUS CELLULOSE; NORMAL-MODES; DYNAMICS; PROTEIN; SPECTROSCOPY; CELLOBIOSE; CRYSTAL; NMR;
D O I
10.1021/jacs.0c09933
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Biomolecules function by adopting multiple conformations. Such dynamics are governed by the conformation landscape whose study requires characterization of the ground and excited conformation states. Here, the conformational landscape of a molecule is sampled by exciting an initial gas-phase molecular conformer into diverse conformation states, using soft molecule-surface collision (0.5-5.0 eV). The resulting ground and excited molecular conformations, adsorbed on the surface, are imaged at the single-molecule level. This technique permits the exploration of oligosaccharide conformations, until now, limited by the high flexibility of oligosaccharides and ensemble-averaged analytical methods. As a model for cellulose, cellohexaose chains are observed in two conformational extremes, the typical "extended" chain and the atypical "coiled" chain-the latter identified as the gas-phase conformer preserved on the surface. Observing conformations between these two extremes reveals the physical properties of cellohexaose, behaving as a rigid ribbon that becomes flexible when twisted. The conformation space of any molecule that can be electrosprayed can now be explored.
引用
收藏
页码:21420 / 21427
页数:8
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