Robust room temperature persistent photoconductivity in polycrystalline indium oxide films

被引:33
作者
Dixit, A. [1 ]
Panguluri, Raghava P. [1 ]
Sudakar, C. [1 ]
Kharel, P. [1 ]
Thapa, P. [1 ]
Avrutsky, I. [1 ,2 ]
Naik, R. [1 ]
Lawes, G. [1 ]
Nadgorny, B. [1 ]
机构
[1] Wayne State Univ, Dept Phys & Astron, Detroit, MI 48201 USA
[2] Wayne State Univ, Dept Elect & Comp Engn, Detroit, MI 48202 USA
基金
美国国家科学基金会;
关键词
carrier density; indium compounds; photoconductivity; semiconductor materials; semiconductor thin films; ultraviolet radiation effects; ultraviolet spectra; visible spectra; ELECTRICAL-PROPERTIES; RELAXATION;
D O I
10.1063/1.3159623
中图分类号
O59 [应用物理学];
学科分类号
摘要
We have investigated the effects of UV irradiation on the electrical and optical properties of polycrystalline In2O3 films. We found that UV illumination at a peak wavelength of 365 nm leads to a sharp drop in resistance and increase in carrier concentration. This highly conductive state persists for a timescale of hours in air at room temperature after illumination. We observe distinct changes in the optical absorption spectra and the associated change in carrier concentration, which is consistent with a Burstein-Moss shift of similar to 0.1 eV. The relaxation rate of this persistent conducting state depends strongly on temperature. We find that the conductance relaxation in an oxygen-free environment can be described by a stretched exponential while the behavior of the samples in air is better described by a logarithmic relaxation, both of which may be associated with glassy behavior.
引用
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页数:3
相关论文
共 19 条
[1]   Deposition and electrical properties of N-In codoped p-type ZnO films by ultrasonic spray pyrolysis [J].
Bian, JM ;
Li, XM ;
Gao, XD ;
Yu, WD ;
Chen, LD .
APPLIED PHYSICS LETTERS, 2004, 84 (04) :541-543
[2]   Growth of In2O3(100) on Y-stabilized ZrO2(100) by O-plasma assisted molecular beam epitaxy [J].
Bourlange, A. ;
Payne, D. J. ;
Egdell, R. G. ;
Foord, J. S. ;
Edwards, P. P. ;
Jones, M. O. ;
Schertel, A. ;
Dobson, P. J. ;
Hutchison, J. L. .
APPLIED PHYSICS LETTERS, 2008, 92 (09)
[3]   THEORY OF THE ATOMIC AND ELECTRONIC-STRUCTURE OF DX CENTERS IN GAAS AND ALXGA1-XAS ALLOYS [J].
CHADI, DJ ;
CHANG, KJ .
PHYSICAL REVIEW LETTERS, 1988, 61 (07) :873-876
[4]   Band structure of indium oxide: Indirect versus direct band gap [J].
Erhart, Paul ;
Klein, Andreas ;
Egdell, Russell G. ;
Albe, Karsten .
PHYSICAL REVIEW B, 2007, 75 (15)
[5]   Indium-oxide polymorphs from first principles: Quasiparticle electronic states [J].
Fuchs, F. ;
Bechstedt, F. .
PHYSICAL REVIEW B, 2008, 77 (15)
[6]   BAND-GAP WIDENING IN HEAVILY SN-DOPED IN2O3 [J].
HAMBERG, I ;
GRANQVIST, CG ;
BERGGREN, KF ;
SERNELIUS, BE ;
ENGSTROM, L .
PHYSICAL REVIEW B, 1984, 30 (06) :3240-3249
[7]  
HARTNAGEL H., 1995, Semiconducting Transparent Thin Films
[8]   STRETCHED-EXPONENTIAL RELAXATION ARISING FROM DISPERSIVE DIFFUSION OF HYDROGEN IN AMORPHOUS-SILICON [J].
KAKALIOS, J ;
STREET, RA ;
JACKSON, WB .
PHYSICAL REVIEW LETTERS, 1987, 59 (09) :1037-1040
[9]  
Kiriakidis G, 2001, PHYS STATUS SOLIDI A, V185, P27, DOI 10.1002/1521-396X(200105)185:1<27::AID-PSSA27>3.0.CO
[10]  
2-U