Long-range transport of Siberian biomass burning emissions and impact on surface ozone in western North America -: art. no. L16106

被引:214
|
作者
Jaffe, D
Bertschi, I
Jaeglé, L
Novelli, P
Reid, JS
Tanimoto, H
Vingarzan, R
Westphal, DL
机构
[1] Univ Washington, Dept Atmospher Sci, Seattle, WA 98011 USA
[2] NOAA, Climate Monitoring & Diagnost Lab, Boulder, CO 80303 USA
[3] USN, Res Lab, Aerosal & Radiat Modeling Sect, Washington, DC 20375 USA
[4] Natl Inst Environm Studies, Div Atmospher Environm, Tsukuba, Ibaraki, Japan
[5] Environm Canada, Aquat & Atmospher Sci Div, Pacific & Yukon Reg, Vancouver, BC, Canada
关键词
D O I
10.1029/2004GL020093
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
During the summer of 2003, biomass fires burned a large area of Siberia, the largest in at least 10 years. We used the NRL Aerosol Analysis and Prediction System (NAAPS) model to forecast the transport of the smoke from these fires. Transport of these airmasses to North America was confirmed by aircraft and surface observations. The fires resulted in enhancements in summer background CO and O-3 of 23 - 37 and 5 - 9 ppbv, respectively, at 10 sites in Alaska, Canada and the Pacific Northwest. From the area burned, we estimate that the Siberian fires generated 68 Tg of CO and 0.82 Tg of NOx ( as N). In addition, we show that the background O-3 enhancement contributed to an exceedance of the ozone air quality standard in the Pacific Northwest. These results show that regional air quality and health are linked to global processes, including climate, forest fires and long-range transport of pollutants.
引用
收藏
页码:L161061 / 4
页数:4
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