Atmospheric transport drives regional interactions of ozone pollution in China

被引:41
|
作者
Shen, Lijuan [1 ,2 ]
Liu, Jane [2 ]
Zhao, Tianliang [1 ]
Xu, Xiangde [3 ]
Han, Han [4 ]
Wang, Honglei [1 ,2 ]
Shu, Zhuozhi [1 ]
机构
[1] Nanjing Univ Informat Sci & Technol, Key Lab Aerosol Cloud Precipitat, China Meteorol Adm, Nanjing 210044, Peoples R China
[2] Univ Toronto, Dept Geog & Planning, Toronto, ON M5S3G3, Canada
[3] China Acad Meteorol Sci, State Key Lab Disastrous Weather, Beijing 100081, Peoples R China
[4] Peking Univ, Sch Phys, Dept Atmospher & Ocean Sci, Lab Climate & Ocean Atmosphere Studies, Beijing 100871, Peoples R China
基金
中国国家自然科学基金;
关键词
Tropospheric ozone; Source-receptor relationship; Transport mechanism; China; FINE PARTICULATE MATTER; TROPOSPHERIC OZONE; SURFACE-OZONE; ANTHROPOGENIC EMISSIONS; SPRINGTIME OZONE; TIBETAN PLATEAU; BOUNDARY-LAYER; AIR-QUALITY; METEOROLOGICAL INFLUENCES; GLOBAL SIMULATION;
D O I
10.1016/j.scitotenv.2022.154634
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In recent years, ozone pollution becomes a serious environmental issue in China. A good understanding of sourcereceptor relationships of ozone transport from aboard and inside China is beneficial to mitigating ozone pollution there. To date, these issues have not been comprehensively assessed, especially for highly polluted regions in the central and eastern China (CEC), including the North China Plain (NCP), Twain-Hu region (THR), Yangtze River Delta (YRD), Pearl River Delta (PRD), and Sichuan Basin (SCB). Here, based on simulations over 2013-2020 from a wellvalidated chemical transport model, GEOS-Chem, we show that foreign ozone accounts for a large portion of surface ozone over CEC, ranging from 25.0% in THR to 39.4% in NCP. Focusing on transport of domestic ozone between the five regions in CEC, we find that atmospheric transport can largely modulate regional interactions of ozone pollution in China. At the surface, THR receives the largest amount of ozone from the other four regions (54.2% of domestic ozone in the receptor region, the same in below), followed by PRD (32.3%), SCB (26.7%), YRD (21.1%), and NCP (18.0%). Meanwhile, YRD exports largest amount of ozone to the other regions, ranging from 8.9% in SCB to 28.4% in THR. Although SCB is relatively isolated and thus impacts NCP, YRD, and PRD weakly (< 2.2%), export of SCB ozone to of (2022) THR reaches 9.3%. The regional ozone transport over CEC, occurring mostly in the lower troposphere, is mainly modulated by the East Asian monsoon circulations, proximity between source and receptor regions, seasonal changes of ozone production, and topography.
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页数:13
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