Ti(3)C(2)Tx MXene aerogel;
SnO2;
Reduced graphene oxide;
Formaldehyde;
Gas sensor;
Room temperature;
GAS SENSOR;
NANOCOMPOSITES;
D O I:
10.1016/j.jallcom.2022.166664
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
The high-performance formaldehyde sensor is an ideal choice for industrial gas detection and environmental gas analysis. In this article, the 3D Ti3C2Tx MXene/rGO/SnO2 aerogle was successfully fabricated via a simple one-step solvothermal route. The composite structures and morphology were characterized by an array of testing techniques. According to the gas measurement, the 3D Ti3C2Tx MXene/rGO/SnO2 sensor exhibited 54.97% sensing response in 10 ppm formaldehyde at room temperature (RT). Not only that, the 3D Ti3C2Tx MXene/rGO/SnO2-based sensor indicated an excellent sensing selectivity, short response and recovery times (2.9 and 2.2 s, separately), good repeatability and stability. A general formaldehyde sensing mechanism with a ternary architectural was proposed and supported through density functional theory (DFT) calculations data, which has been sufficiently shown to be a promising candidate for the design of efficient formaldehyde sensor. (c) 2022 Elsevier B.V. All rights reserved.
机构:
Northwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R ChinaNorthwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R China
Xu, Xiaoli
Jiang, Hongtao
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Northwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R ChinaNorthwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R China
Jiang, Hongtao
Liu, Wangwang
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Northwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R ChinaNorthwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R China
Liu, Wangwang
Wang, Shengyi
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机构:
Southwest Univ, Sch Mat & Energy, Chongqing 400715, Peoples R ChinaNorthwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R China
Wang, Shengyi
Wang, Xiaoping
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机构:
Nankai Univ, Coll Environm Sci & Engn, Tianjin 300350, Peoples R ChinaNorthwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R China
Wang, Xiaoping
Wang, Mengyu
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机构:
Northwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R ChinaNorthwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R China
Wang, Mengyu
Ma, Wei
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Northwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R ChinaNorthwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R China
Ma, Wei
Sun, Guorong
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Northwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R ChinaNorthwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R China
Sun, Guorong
Liu, Jiming
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Northwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R ChinaNorthwest Normal Univ, Coll Phys & Elect Engn, Key Lab Atom & Mol Phys & Funct Mat Gansu Prov, Lanzhou 730070, Peoples R China
机构:
East China Univ Sci & Technol, MOE Key Lab Pressure Syst & Safety, Shanghai 200237, Peoples R China
East China Univ Sci & Technol, Sch Mech & Power Engn, Shanghai 200237, Peoples R ChinaEast China Univ Sci & Technol, MOE Key Lab Pressure Syst & Safety, Shanghai 200237, Peoples R China
Wang, Lei
Xiao, Zhikun
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East China Univ Sci & Technol, MOE Key Lab Pressure Syst & Safety, Shanghai 200237, Peoples R China
East China Univ Sci & Technol, Sch Mech & Power Engn, Shanghai 200237, Peoples R ChinaEast China Univ Sci & Technol, MOE Key Lab Pressure Syst & Safety, Shanghai 200237, Peoples R China
Xiao, Zhikun
Yao, Xinqi
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East China Univ Sci & Technol, MOE Key Lab Pressure Syst & Safety, Shanghai 200237, Peoples R China
East China Univ Sci & Technol, Sch Mech & Power Engn, Shanghai 200237, Peoples R ChinaEast China Univ Sci & Technol, MOE Key Lab Pressure Syst & Safety, Shanghai 200237, Peoples R China
Yao, Xinqi
Yu, Xinhai
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机构:
East China Univ Sci & Technol, MOE Key Lab Pressure Syst & Safety, Shanghai 200237, Peoples R China
East China Univ Sci & Technol, Sch Mech & Power Engn, Shanghai 200237, Peoples R ChinaEast China Univ Sci & Technol, MOE Key Lab Pressure Syst & Safety, Shanghai 200237, Peoples R China
Yu, Xinhai
Tu, Shan-Tung
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机构:
East China Univ Sci & Technol, MOE Key Lab Pressure Syst & Safety, Shanghai 200237, Peoples R China
East China Univ Sci & Technol, Sch Mech & Power Engn, Shanghai 200237, Peoples R ChinaEast China Univ Sci & Technol, MOE Key Lab Pressure Syst & Safety, Shanghai 200237, Peoples R China
Tu, Shan-Tung
Chen, Shijian
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机构:
SUFA Technol Ind Co Ltd, CNNC, Suzhou 215001, Peoples R ChinaEast China Univ Sci & Technol, MOE Key Lab Pressure Syst & Safety, Shanghai 200237, Peoples R China