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3D porous Ti3C2Tx MXene/rGO/SnO2 aerogel for formaldehyde detection at room temperature
被引:20
|作者:
Liu, Miao
[1
]
Song, Peng
[1
]
Liang, Dong
[1
]
Ding, Yongling
[2
]
Wang, Qi
[1
]
机构:
[1] Univ Jinan, Sch Mat Sci & Engn, Jinan 250022, Peoples R China
[2] Shandong Jiaotong Univ, Sch Transportat Civil Engn, Jinan 250357, Peoples R China
基金:
中国国家自然科学基金;
关键词:
Ti(3)C(2)Tx MXene aerogel;
SnO2;
Reduced graphene oxide;
Formaldehyde;
Gas sensor;
Room temperature;
GAS SENSOR;
NANOCOMPOSITES;
D O I:
10.1016/j.jallcom.2022.166664
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
The high-performance formaldehyde sensor is an ideal choice for industrial gas detection and environmental gas analysis. In this article, the 3D Ti3C2Tx MXene/rGO/SnO2 aerogle was successfully fabricated via a simple one-step solvothermal route. The composite structures and morphology were characterized by an array of testing techniques. According to the gas measurement, the 3D Ti3C2Tx MXene/rGO/SnO2 sensor exhibited 54.97% sensing response in 10 ppm formaldehyde at room temperature (RT). Not only that, the 3D Ti3C2Tx MXene/rGO/SnO2-based sensor indicated an excellent sensing selectivity, short response and recovery times (2.9 and 2.2 s, separately), good repeatability and stability. A general formaldehyde sensing mechanism with a ternary architectural was proposed and supported through density functional theory (DFT) calculations data, which has been sufficiently shown to be a promising candidate for the design of efficient formaldehyde sensor. (c) 2022 Elsevier B.V. All rights reserved.
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