Pyroelectric and dielectric properties of sol-gel derived barium-strontium-titanate (Ba0.64Sr0.36TiO3) thin films

被引:36
作者
Zhang, TJ [1 ]
Ni, H [1 ]
机构
[1] Hubei Univ, Sch Phys & Elect Technol, Wuhan 430062, Peoples R China
关键词
BST thin films; dielectric and pyroelectric properties; capacitance-frequency curve; material figure-of-merit; sol-gel process;
D O I
10.1016/S0924-4247(02)00139-5
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
The barium-strontium-titanate (BST, Ba0(.64)Sr(0.36)TiO(3)) thin films have been prepared by the sol-gel method on a platinum-coated silicon substrate. The resulting thin films show very good dielectric and pyroelectric properties. The dielectric constant and dissipation factor for Ba0.64Sr0.36TiO3 thin film at a frequency of 200 Hz were 592 and 0.028, respectively. The dependence of the capacitance as a function of the voltage shows a strongly non-linear character, and two peaks characterizing spontaneous polarization switching can be clearly seen in this curve, indicating that the films have a ferroelectric nature. The capacitance changed from 495 to 1108 pF with the applied voltage in the -5 to +5 V range at a frequency of 100 kHz. The peak pyroelectric coefficient at 30 degreesC is 1080 muC/m(2) K. The pyroelectric coefficient at room temperature (25 degreesC) is 1860 muC/m(2) K, and the figure-of-merit of this film is 37.4 muC/m(3). The high pyroelectric coefficients and the greater figures-of-merit of Ba0.64Sr0.36TiO3 thin films make it possible to be used for thermal infrared detection and imaging. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:252 / 256
页数:5
相关论文
共 11 条
[1]   PYROELECTRIC COEFFICIENT DIRECT MEASUREMENT TECHNIQUE AND APPLICATION TO A NSEC RESPONSE TIME DETECTOR [J].
BYER, RL ;
ROUNDY, CB .
IEEE TRANSACTIONS ON SONICS AND ULTRASONICS, 1972, SU19 (02) :333-&
[2]   PREPARATION OF BARIUM STRONTIUM-TITANATE THIN-FILM CAPACITORS ON SILICON BY METALLORGANIC DECOMPOSITION [J].
CATALAN, AB ;
MANTESE, JV ;
MICHELI, AL ;
SCHUBRING, NW ;
POISSON, RJ .
JOURNAL OF APPLIED PHYSICS, 1994, 76 (04) :2541-2543
[3]   DIELECTRIC-PROPERTIES OF (BA, SR)TIO3 THIN-FILMS DEPOSITED BY RF-SPUTTERING [J].
HORIKAWA, T ;
MIKAMI, N ;
MAKITA, T ;
TANIMURA, J ;
KATAOKA, M ;
SATO, K ;
NUNOSHITA, M .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS SHORT NOTES & REVIEW PAPERS, 1993, 32 (9B) :4126-4130
[4]   Dielectric properties of sol-gel derived barium-strontium-titanate (Ba0.4Sr0.6TiO3) thin films [J].
Lahiry, S ;
Gupta, V ;
Sreenivas, K ;
Mansingh, A .
IEEE TRANSACTIONS ON ULTRASONICS FERROELECTRICS AND FREQUENCY CONTROL, 2000, 47 (04) :854-860
[5]  
LINES ME, 1997, PRINCIPLES APPL FERR, P620
[6]   Pyroelectric infrared arrays and their applications [J].
Norkus, V ;
Sokoll, T ;
Gerlach, G ;
Hofmann, G .
INFRARED SPACEBORNE REMOTE SENSING V, 1997, 3122 :409-419
[7]   PBTIO3 FERROELECTRIC THIN-FILMS AND THEIR PYROELECTRIC APPLICATION [J].
OKUYAMA, M ;
HAMAKAWA, Y .
FERROELECTRICS, 1991, 118 (1-4) :261-278
[8]   Dielectric response in pulsed laser ablated (Ba,Sr)TiO3 thin films [J].
Saha, S ;
Krupanidhi, SB .
JOURNAL OF APPLIED PHYSICS, 2000, 87 (02) :849-854
[9]  
Sengupta L. C., 1998, Integrated Ferroelectrics, V22, P393, DOI 10.1080/10584589808208059
[10]   STRUCTURAL AND ELECTRICAL-PROPERTIES OF RF-SPUTTERED AMORPHOUS BARIUM-TITANATE THIN-FILMS [J].
SREENIVAS, K ;
MANSINGH, A ;
SAYER, M .
JOURNAL OF APPLIED PHYSICS, 1987, 62 (11) :4475-4481