Effect of extreme pump pulse reshaping on intense terahertz emission in lithium niobate at multimilliJoule pump energies

被引:56
作者
Blanchard, F. [1 ]
Ropagnol, X. [2 ]
Hafez, H. [2 ]
Razavipour, H. [1 ]
Bolduc, M. [3 ]
Morandotti, R. [2 ]
Ozaki, T. [2 ]
Cooke, D. G. [1 ]
机构
[1] McGill Univ, Dept Phys, Quebec City, PQ H3A 2TB, Canada
[2] Inst Natl Rech Sci INRS EMT, Varennes, PQ J3X 1S2, Canada
[3] INO Quebec, Quebec City, PQ G1P 4S4, Canada
基金
加拿大自然科学与工程研究理事会;
关键词
OPTICAL RECTIFICATION; THZ PULSES; GENERATION; LINBO3;
D O I
10.1364/OL.39.004333
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We report on terahertz (THz) generation via optical rectification in a room-temperature lithium niobate crystal under variable pump pulse durations, ranging from 100 to 300 fs, at 800 nm center wavelength. The efficiency for the process is predicted to have an order of magnitude increase when longer duration Fourier-limited pump pulses are used. Our results confirm this increase in efficiency, and we report a record 800 nm pump energy conversion efficiency of 0.35% with a saturation at >240 fs pulse duration. While promising, our findings show a series of key problems that must be overcome before the theoretical limit can be achieved, including the influence of the pump bandwidth broadening due to the cascaded nonlinearity taking place within the crystal. (C) 2014 Optical Society of America
引用
收藏
页码:4333 / 4336
页数:4
相关论文
共 23 条
[1]   Generation of 1.5 μJ single-cycle terahertz pulses by optical rectification from a large aperture ZnTe crystal [J].
Blanchard, F. ;
Razzari, L. ;
Bandulet, H.-C. ;
Sharma, G. ;
Morandotti, R. ;
Kieffer, J.-C. ;
Ozaki, T. ;
Reid, M. ;
Tiedje, H. F. ;
Haugen, H. K. ;
Hegmann, F. A. .
OPTICS EXPRESS, 2007, 15 (20) :13212-13220
[2]   Real-time terahertz near-field microscope [J].
Blanchard, F. ;
Doi, A. ;
Tanaka, T. ;
Hirori, H. ;
Tanaka, H. ;
Kadoya, Y. ;
Tanaka, K. .
OPTICS EXPRESS, 2011, 19 (09) :8277-8284
[3]   Terahertz generation by tilted-front laser pulses in weakly and strongly nonlinear regimes [J].
Bodrov, Sergey B. ;
Murzanev, Aleksey A. ;
Sergeev, Yury A. ;
Malkov, Yury A. ;
Stepanov, Andrey N. .
APPLIED PHYSICS LETTERS, 2013, 103 (25)
[4]  
Bolduc M., 2013, P INT C INFR MILL TE, P1
[5]   Cascaded nonlinear difference-frequency generation of enhanced terahertz wave production [J].
Cronin-Golomb, M .
OPTICS LETTERS, 2004, 29 (17) :2046-2048
[6]   Generation of sub-mJ terahertz pulses by optical rectification [J].
Fueloep, J. A. ;
Palfalvi, L. ;
Klingebiel, S. ;
Almasi, G. ;
Krausz, F. ;
Karsch, S. ;
Hebling, J. .
OPTICS LETTERS, 2012, 37 (04) :557-559
[7]   Towards generation of mJ-level ultrashort THz pulses by optical rectification [J].
Fueloep, Jozsef Andras ;
Palfalvi, Laszlo ;
Hoffmann, Matthias C. ;
Hebling, Janos .
OPTICS EXPRESS, 2011, 19 (16) :15090-15097
[8]   Nonlinear terahertz response of n-type GaAs [J].
Gaal, P. ;
Reimann, K. ;
Woerner, M. ;
Elsaesser, T. ;
Hey, R. ;
Ploog, K. H. .
PHYSICAL REVIEW LETTERS, 2006, 96 (18)
[9]   Velocity matching by pulse front tilting for large-area THz-pulse generation [J].
Hebling, J ;
Almási, G ;
Kozma, IZ ;
Kuhl, J .
OPTICS EXPRESS, 2002, 10 (21) :1161-1166
[10]   Single-cycle terahertz pulses with amplitudes exceeding 1 MV/cm generated by optical rectification in LiNbO3 [J].
Hirori, H. ;
Doi, A. ;
Blanchard, F. ;
Tanaka, K. .
APPLIED PHYSICS LETTERS, 2011, 98 (09)