SO2 Removal in a Pilot Scale Rotating Packed Bed

被引:18
作者
Bai, Shun [1 ,2 ]
Chu, Guang-Wen [1 ,2 ]
Li, Shao-Chen [2 ]
Zou, Hai-Kui [2 ]
Xiang, Yang [2 ]
Luo, Yong [2 ]
Chen, Jian-Feng [1 ,2 ]
机构
[1] Beijing Univ Chem Technol, State Key Lab Organ Inorgan Composites, Beijing 100029, Peoples R China
[2] Beijing Univ Chem Technol, Res Ctr, Minist Educ High Grav Engn & Technol, Beijing 100029, Peoples R China
基金
中国国家自然科学基金;
关键词
desulfurization; plastic packing; rotating packed bed; structured SiC packing; FLUE-GAS DESULFURIZATION; MASS-TRANSFER; PROCESS INTENSIFICATION; DISTILLATION; TECHNOLOGY; ABSORPTION; PACKING; AREA;
D O I
10.1089/ees.2014.0412
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Absorption of SO2 from a gas mixture with an ammonia-based solution was investigated using a counter current rotating packed bed (RPB) with SiC structured packing and plastic packing. Effects of operating parameters, such as the rotational speed, liquid flow rate, gas flow rate, liquid-gas ratio, inlet concentration of SO2, and the alkalinity of absorbent on the removal efficiency of SO2, were examined. Experimental results showed that the plastic packing had a better desulfurization performance under the same operation conditions. Moreover, correlations of gas-side volumetric overall mass transfer coefficients of the RPB with the two types of packing were obtained and the predicted data were in good agreement with experimental results.
引用
收藏
页码:806 / 815
页数:10
相关论文
共 35 条
[1]   Flue gas desulfurization by citrate process and optimization of working parameters [J].
Akyalcin, L. ;
Kaytakoglu, S. .
CHEMICAL ENGINEERING AND PROCESSING-PROCESS INTENSIFICATION, 2010, 49 (02) :199-204
[2]   Synthesis of nanoparticles with novel technology: High-gravity reactive precipitation [J].
Chen, JF ;
Wang, YH ;
Guo, F ;
Wang, XM ;
Zheng, C .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2000, 39 (04) :948-954
[3]   Packing characteristics for mass transfer in a rotating packed bed [J].
Chen, Yu-Shao ;
Lin, Fang-Yi ;
Lin, Chia-Chang ;
Tai, Clifford Yi-Der ;
Liu, Hwai-Shen .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2006, 45 (20) :6846-6853
[4]   Flue gas desulfurization in an internally circulating fluidized bed reactor [J].
Chu, CY ;
Hwang, SJ .
POWDER TECHNOLOGY, 2005, 154 (01) :14-23
[5]   Absorption of SO2 with Ammonia-Based Solution in a Cocurrent Rotating Packed Bed [J].
Chu, Guang-Wen ;
Luo, Yong ;
Shan, Cong-Yun ;
Zou, Hai-Kui ;
Xiang, Yang ;
Shao, Lei ;
Chen, Jian-Feng .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2014, 53 (40) :15731-15737
[6]   Distillation studies in a two-stage counter-current rotating packed bed [J].
Chu, Guang-Wen ;
Gao, Xin ;
Luo, Yong ;
Zou, Hai-Kui ;
Shao, Lei ;
Chen, Jian-Feng .
SEPARATION AND PURIFICATION TECHNOLOGY, 2013, 102 :62-66
[7]   Prediction of SO2 removal efficiency for wet Flue Gas Desulfurization [J].
Dou, Binlin ;
Pan, Weiguo ;
Jin, Qiang ;
Wang, Wenhuan ;
Li, Yu .
ENERGY CONVERSION AND MANAGEMENT, 2009, 50 (10) :2547-2553
[8]   Gas-liquid absorption reaction between (NH4)2SO3 solution and SO2 for ammonia-based wet flue gas desulfurization [J].
Gao, Xiang ;
Ding, Honglei ;
Du, Zhen ;
Wu, Zuliang ;
Fang, Mengxiang ;
Luo, Zhongyang ;
Cen, Kefa .
APPLIED ENERGY, 2010, 87 (08) :2647-2651
[9]   Optimal Packing of a Rotating Packed Bed for H2S Removal [J].
Guo, Kai ;
Wen, Jiawu ;
Zhao, Ying ;
Wang, Yu ;
Zhang, Zhenzhen ;
Li, Zongxiang ;
Qian, Zhi .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2014, 48 (12) :6844-6849
[10]   An Innovative Approach of the Effective Mass Transfer Area in the Rotating Packed Bed [J].
Guo, Kai ;
Zhang, Zhenzhen ;
Luo, Huijuan ;
Dang, Jiaxi ;
Qian, Zhi .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2014, 53 (10) :4052-4058