High-efficient synergy of piezocatalysis and photocatalysis in bismuth oxychloride nanomaterial for dye decomposition

被引:164
作者
Ismail, Muhammad [1 ,2 ,4 ]
Wu, Zheng [1 ,2 ]
Zhang, Luohong [1 ]
Ma, Jiangping [4 ]
Jia, Yanmin [3 ,4 ]
Hu, Yongming [5 ]
Wang, Yaojin [6 ]
机构
[1] Xian Polytech Univ, Sch Environm & Chem Engn, Xian 710048, Shaanxi, Peoples R China
[2] Zhejiang Normal Univ, Coll Geog & Environm Sci, Jinhua 321004, Zhejiang, Peoples R China
[3] Xian Univ Posts & Telecommun, Sch Sci, Xian 710121, Shaanxi, Peoples R China
[4] Zhejiang Normal Univ, Dept Phys, Jinhua 321004, Zhejiang, Peoples R China
[5] Hubei Univ, Fac Phys & Elect Sci, Hubei Key Lab Ferro & Piezoelect Mat & Devices, Wuhan 430062, Hubei, Peoples R China
[6] Nanjing Univ Sci & Technol, Sch Mat Sci & Engn, Nanjing 210094, Jiangsu, Peoples R China
基金
中国国家自然科学基金;
关键词
Piezoelectric effect; Piezocatalysis; Synergy of bi-catalysis; Bismuth oxychloride; Photocatalysis; Dye decomposition; BATIO3; NANOFIBERS; AQUEOUS-SOLUTION; CATALYSIS; REMOVAL; BIOCL; NANOPARTICLES; DEGRADATION; AU; ADSORPTION; POLLUTANTS;
D O I
10.1016/j.chemosphere.2019.04.121
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In this work, it is found that the hydrothermally-synthesized bismuth oxychloride can behave both the piezocatalysis and photocatalysis for the Rhodamine B dye decomposition. similar to 99% decomposition efficiency is achieved after both vibrating and lighting the Rhodamine B dye solution for similar to 96 min with the addition of bismuth oxychloride catalyst, while the similar to 72% and similar to 26% decomposition efficiencies are obtained for only photocatalysis or only piezocatalysis respectively. In bi-catalysis, the mechanical strain produced due to vibration will directly provide an electric field that will increase the separation between the photo-induced electron-hole pairs, yielding to the enhanced decomposition performance of bicatalysis. There is no significant change in the bi-catalytic performance of bismuth oxychloride nanomaterial observed after being recycled four times. Bismuth oxychloride catalyst is potential for the bi-catalytic decomposition treatment of wastewater through harvesting both the environmental vibration energy and light energy. (C) 2019 Elsevier Ltd. All rights reserved.
引用
收藏
页码:212 / 218
页数:7
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