Fugitive Road Dust PM2.5 Emissions and Their Potential Health Impacts

被引:113
作者
Chen, Siyu [1 ]
Zhang, Xiaorui [1 ]
Lin, Jintai [2 ]
Huang, Jianping [1 ]
Zhao, Dan [1 ]
Yuan, Tiangang [1 ]
Huang, Kangning [3 ]
Luo, Yuan [1 ]
Jia, Zhuo [4 ]
Zang, Zhou [1 ]
Qiu, Yue'an [5 ,6 ]
Xie, Li [7 ]
机构
[1] Lanzhou Univ, Minist Educ, Key Lab Semiarid Climate Change, Lanzhou 730000, Gansu, Peoples R China
[2] Peking Univ, Sch Phys, Dept Atmospher & Ocean Sci, Lab Climate & Ocean Atmosphere Studies, Beijing 100871, Peoples R China
[3] Yale Univ, Yale Sch Forestry & Environm Studies, New Haven, CT 06511 USA
[4] Lanzhou Univ, Coll Earth & Environm Sci, Lanzhou 730000, Gansu, Peoples R China
[5] Sun Yat Sen Univ, Sch Geog & Planning, Guangzhou 510275, Guangdong, Peoples R China
[6] Sun Yat Sen Univ, Guangdong Key Lab Urbanizat & Geosimulat, Guangzhou 510275, Guangdong, Peoples R China
[7] Gansu Prov Matern & Child Care Hosp, Lanzhou 730050, Gansu, Peoples R China
基金
中国国家自然科学基金;
关键词
POLYCYCLIC AROMATIC-HYDROCARBONS; AIR-POLLUTION; PARTICULATE MATTER; URBAN FUNCTION; GLOBAL BURDEN; PM10; RISK; INVENTORY; PARTICLES; EXPOSURE;
D O I
10.1021/acs.est.9b00666
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Fugitive road dust (FRD) particles emitted by traffic-generated turbulence are an important contributor to urban ambient fine particulate matter (PM2.5). Especially in urban areas of developing countries, FRD PM2.5 emissions are a serious environmental threat to air quality and public health. FRD PM2.5 emissions have been neglected or substantially underestimated in previous study, resulting in the underestimation of modeling PM concentrations and estimating their health impacts. This study constructed the FRD PM2.5 emissions inventory in a major inland city in China (Lanzhou) in 2017 at high-resolution (500 X 500 m(2)), investigated the spatiotemporal characteristics of the FRD emissions in different urban function zones, and quantified their health impacts. The FRD PM2.5 emission was approximately 1141 +/- 71 kg d(-1), accounting for 24.6% of total PM2.5 emission in urban Lanzhou. Spatially, high emissions exceeding 3 x 10(4) mu g m(-2 )d(-1) occurred over areas with smaller particle sizes, larger traffic intensities, and more frequent construction activities. The estimated premature mortality burden induced by FRD PM2.5 exposure was 234.5 deaths in Lanzhou in 2017. Reducing FRD emissions are an important step forward to protect public health in many developing urban regions.
引用
收藏
页码:8455 / 8465
页数:11
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