Chemistry of Atmospheric Nucleation: On the Recent Advances on Precursor Characterization and Atmospheric Cluster Composition in Connection with Atmospheric New Particle Formation

被引:248
作者
Kulmala, M. [1 ]
Petaja, T. [1 ]
Ehn, M. [1 ,2 ]
Thornton, J. [3 ]
Sipila, M. [1 ]
Worsnop, D. R. [1 ,4 ]
Kerminen, V. -M. [1 ]
机构
[1] Univ Helsinki, Dept Phys, FI-00014 Helsinki, Finland
[2] Inst Energy & Climate Res IEK 8, D-52425 Julich, Germany
[3] Univ Washington, Dept Atmospher Sci, Seattle, WA 98195 USA
[4] Aerodyne Res Inc, Billerica, MA 01821 USA
来源
ANNUAL REVIEW OF PHYSICAL CHEMISTRY, VOL 65 | 2014年 / 65卷
关键词
atmosphere; aerosol formation; cluster dynamics; sulfuric acid; organic compounds; volatility; CLOUD CONDENSATION NUCLEI; STABILIZED CRIEGEE INTERMEDIATE; ORGANIC AEROSOL FORMATION; GALACTIC COSMIC-RAYS; SULFURIC-ACID; BOREAL FOREST; MASS-SPECTROMETER; NEUTRAL CLUSTER; ION NUCLEATION; GROWTH-RATES;
D O I
10.1146/annurev-physchem-040412-110014
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The recent development in measurement techniques and theoretical understanding has enabled us to study atmospheric vapor, cluster and nanoparticle concentrations, dynamics, and their connection to atmospheric nucleation. Here we present a summary of the chemistry of atmospheric clustering, growing nanoparticles, and their precursors. In this work, we focus particularly on atmospheric gas-to-particle conversion and recent progress in its understanding.
引用
收藏
页码:21 / 37
页数:17
相关论文
共 125 条
[1]  
Almeida J, 2013, NATURE UNPUB
[2]  
[Anonymous], ATMOS CHEM PHYS DISC
[3]   ION NUCLEATION - A POTENTIAL SOURCE FOR STRATOSPHERIC AEROSOLS [J].
ARNOLD, F .
NATURE, 1982, 299 (5879) :134-137
[4]   Hygroscopicity and chemical composition of Antarctic sub-micrometre aerosol particles and observations of new particle formation [J].
Asmi, E. ;
Frey, A. ;
Virkkula, A. ;
Ehn, M. ;
Manninen, H. E. ;
Timonen, H. ;
Tolonen-Kivimaki, O. ;
Aurela, M. ;
Hillamo, R. ;
Kulmala, M. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2010, 10 (09) :4253-4271
[5]   Laboratory study on new particle formation from the reaction OH + SO2: influence of experimental conditions, H2O vapour, NH3 and the amine tert-butylamine on the overall process [J].
Berndt, T. ;
Stratmann, F. ;
Sipilae, M. ;
Vanhanen, J. ;
Petaja, T. ;
Mikkila, J. ;
Gruener, A. ;
Spindler, G. ;
Mauldin, R. Lee, III ;
Curtius, J. ;
Kulmala, M. ;
Heintzenberg, J. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2010, 10 (15) :7101-7116
[6]   Gas-Phase Ozonolysis of Selected Olefins: The Yield of Stabilized Criegee Intermediate and the Reactivity toward SO2 [J].
Berndt, Torsten ;
Jokinen, Tuija ;
Mauldin, Roy L., III ;
Petaja, Tuukka ;
Herrmann, Hartmut ;
Junninen, Heikki ;
Paasonen, Pauli ;
Worsnop, Douglas R. ;
Sipila, Mikko .
JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2012, 3 (19) :2892-2896
[7]   A field-deployable, chemical ionization time-of-flight mass spectrometer [J].
Bertram, T. H. ;
Kimmel, J. R. ;
Crisp, T. A. ;
Ryder, O. S. ;
Yatavelli, R. L. N. ;
Thornton, J. A. ;
Cubison, M. J. ;
Gonin, M. ;
Worsnop, D. R. .
ATMOSPHERIC MEASUREMENT TECHNIQUES, 2011, 4 (07) :1471-1479
[8]   Oxidation of SO2 by stabilized Criegee intermediate (sCI) radicals as a crucial source for atmospheric sulfuric acid concentrations [J].
Boy, M. ;
Mogensen, D. ;
Smolander, S. ;
Zhou, L. ;
Nieminen, T. ;
Paasonen, P. ;
Plass-Duelmer, C. ;
Sipila, M. ;
Petaja, T. ;
Mauldin, L. ;
Berresheim, H. ;
Kulmala, M. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2013, 13 (07) :3865-3879
[9]   Amine exchange into ammonium bisulfate and ammonium nitrate nuclei [J].
Bzdek, B. R. ;
Ridge, D. P. ;
Johnston, M. V. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2010, 10 (08) :3495-3503
[10]  
Calvert J. G., 2000, MECH ATMOSPHERIC OXI