Concept for a new cloud condensation nucleus (CCN) spectrometer

被引:7
|
作者
VanReken, TM
Nenes, A
Flagan, RC
Seinfeld, JH
机构
[1] CALTECH, Dept Chem Engn, Pasadena, CA 91125 USA
[2] Georgia Inst Technol, Sch Earth & Atmospher Sci, Atlanta, GA 30332 USA
[3] Georgia Inst Technol, Sch Chem & Biol Engn, Atlanta, GA 30332 USA
关键词
D O I
10.1080/02786820460479842
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
The concept of a new cloud condensation nucleus (CCN) spectrometer based on modifications to the original design of Fukuta and Saxena is presented. The key modifications include introducing a trapezoidal geometry and orienting the chamber vertically. A series of simulations demonstrate the broadening of the effective range of the instrument to include supersaturations lower than those reported for the original instrument, without reducing the maximum resolvable supersaturation. A design criterion is developed to eliminate configurations that would result in secondary flows in the growth chamber resulting from buoyancy effects. Using instrument configurations that satisfy this criterion, the effects of variations in the chamber geometry, the imposed temperature gradient, and the total volumetric flow are evaluated. A new configuration is identified that could produce real-time CCN spectra with an effective range at least including supersaturations between 0.07% and 1.2%.
引用
收藏
页码:639 / 654
页数:16
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