Possible evidence of Coulomb explosion in the femtosecond laser ablation of metal at low laser fluence

被引:33
作者
Li, Shuchang [1 ,2 ]
Li, Suyu [1 ,2 ]
Zhang, Fangjian [1 ,2 ]
Tian, Dan [1 ,2 ]
Li, He [1 ,2 ]
Liu, Dunli [1 ,2 ]
Jiang, Yuanfei [1 ,2 ]
Chen, Anmin [1 ,2 ]
Jin, Mingxing [1 ,2 ]
机构
[1] Jilin Univ, Inst Atom & Mol Phys, Changchun 130012, Peoples R China
[2] Jilin Univ, Jilin Prov Key Lab Appl Atom & Mol Spect, Changchun 130012, Peoples R China
基金
中国博士后科学基金; 中国国家自然科学基金;
关键词
Coulomb explosion; Femtosecond laser; Ablation; THERMIONIC EMISSION; THERMAL-MODEL; PHASE-CHANGE; COPPER;
D O I
10.1016/j.apsusc.2015.07.136
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We use a computational model to study the ablation mechanism of metal target irradiated by femtosecond pulse laser. It is confirmed that the Coulomb explosion can occur during femtosecond laser ablation of metal. The influence of thermal ablation and Coulomb explosion on the ablation depth is respectively investigated. Comparing the calculated results with the experimental ones, we find that the theoretical results which consider the thermal ablation only agree well with the experimental ones at high laser fluence, and those which take the Coulomb explosion into account fit well with the experimental ones at lower laser fluence, which exactly explains the ablation mechanism. In contrast with the previous theoretical results which only consider the thermal ablation, our theoretical simulation describes the ablation mechanism straightforward by making comparison of ablation depth, and provides a more reasonable explanation that fits with the actual ablation process. (C) 2015 Elsevier B.V. All rights reserved.
引用
收藏
页码:681 / 685
页数:5
相关论文
共 35 条
[1]  
[Anonymous], 2004, CRC Handbook of Chemistry and Physics, V84th, P2475
[2]   Subpicosecond laser ablation of copper and fused silica: Initiation threshold and plasma expansion [J].
Axente, E. ;
Noel, S. ;
Hermann, J. ;
Sentis, M. ;
Mihailescu, I. N. .
APPLIED SURFACE SCIENCE, 2009, 255 (24) :9734-9737
[3]   Simulation of the thermionic emission during ultrashort pulse laser ablation of metals [J].
Balasubramani, T. ;
Jeong, S. H. .
COLA'05: 8TH INTERNATIONAL CONFERENCE ON LASER ABLATION, 2007, 59 :595-+
[4]   Enhanced two temperature modeling of ultrashort laser ablation for the investigation of thermionic emission characteristics [J].
Balasubramni, T. ;
Kim, S. H. ;
Jeong, S. H. .
APPLIED SURFACE SCIENCE, 2009, 255 (24) :9601-9604
[5]   Energy balance of pulsed laser ablation: thermal model revised [J].
Bulgakova, NM ;
Bulgakov, AV ;
Babich, LP .
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 2004, 79 (4-6) :1323-1326
[6]   Electronic transport and consequences for material removal in ultrafast pulsed laser ablation of materials [J].
Bulgakova, NM ;
Stoian, R ;
Rosenfeld, A ;
Hertel, IV ;
Campbell, EEB .
PHYSICAL REVIEW B, 2004, 69 (05)
[7]   Thermal behavior of thin metal films irradiated by shaped femtosecond pulse sequences laser [J].
Chen, A. M. ;
Jiang, Y. F. ;
Sui, L. Z. ;
Ding, D. J. ;
Liu, H. ;
Jin, M. X. .
OPTICS COMMUNICATIONS, 2011, 284 (08) :2192-2197
[8]   Thrust enhancement via gel-type liquid confinement of laser ablation of solid metal propellant [J].
Choi, Soojin ;
Han, Tae-hee ;
Gojani, Ardian B. ;
Yoh, Jack J. .
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 2010, 98 (01) :147-151
[9]   Ultra-short laser ablation of metals and semiconductors: evidence of ultra-fast Coulomb explosion [J].
Dachraoui, H ;
Husinsky, W ;
Betz, G .
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 2006, 83 (02) :333-336
[10]   Fast electronic and thermal processes in femtosecond laser ablation of Au [J].
Dachraoui, Hatem ;
Husinsky, Wolfgang .
APPLIED PHYSICS LETTERS, 2006, 89 (10)