Green removal of pyridine from water via adsolubilization with lignosulfonate intercalated layered double hydroxide

被引:19
作者
Xia, Mengqi [1 ]
Jin, Cheng [1 ]
Kong, Xianggui [1 ]
Jiang, Meihong [1 ]
Lei, Deqiang [2 ]
Lei, Xiaodong [1 ]
机构
[1] Beijing Univ Chem Technol, Beijing, Peoples R China
[2] Huazhong Univ Sci & Technol, Wuhan, Hubei, Peoples R China
基金
中国国家自然科学基金;
关键词
Adsorption; wastewater treatment; adsolubilization; layered double hydroxide; regeneration; IMMOBILIZED PIMELOBACTER SP; AQUEOUS-SOLUTION; ADSORPTION BEHAVIOR; BIODEGRADATION; HYDROTALCITE; DERIVATIVES; ADSORBENT; CO32;
D O I
10.1177/0263617417737642
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
In this work, lignosulfonate intercalated Mg2Al layered double hydroxide was fabricated by coprecipitation method, which was used as a functional adsorbent for removing pyridine from wastewater. The X-ray powder diffraction and Fourier transformed infrared were carried out to investigate the structure of the product. In the removal process, the as-prepared lignosulfonate intercalated Mg2Al layered double hydroxide sample exhibited good adsolubilization property for pyridine, with maximum capacity of 400.8 mg g(-1) in initial pyridine concentration of 400 mg/l and the removal percentage achieved about 87.9%. In addition, the influence of pH, time, and initial concentration of pyridine on the adsorption capacity was also examined. Moreover, the adsorption kinetic followed the pseudo-second-order model. Furthermore, after regeneration, the adsorbent can still show high adsorption capacity even for 10 cycles of desorption-adsorption. It hoped that lignosulfonate intercalated Mg2Al layered double hydroxide can be used as adsorbent for the removal of organic pollutants in wastewater.
引用
收藏
页码:982 / 998
页数:17
相关论文
共 44 条
[1]   Lignocellulosic-derived modified agricultural waste: Development, characterisation and implementation in sequestering pyridine from aqueous solutions [J].
Ahmed, Md Juned K. ;
Ahmaruzzaman, M. ;
Reza, Ruhul A. .
JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2014, 428 :222-234
[2]   Removal of Pyridine from Aqueous Solution by Adsorption on an Activated Carbon Cloth [J].
Alonso-Davila, Pedro ;
Torres-Rivera, Oliva L. ;
Leyva-Ramos, Roberto ;
Ocampo-Perez, Raul .
CLEAN-SOIL AIR WATER, 2012, 40 (01) :45-53
[3]   OZONATION OF PYRIDINE IN AQUEOUS-SOLUTION - MECHANISTIC AND KINETIC ASPECTS [J].
ANDREOZZI, R ;
INSOLA, A ;
CAPRIO, V ;
DAMORE, MG .
WATER RESEARCH, 1991, 25 (06) :655-659
[4]   Optical and Thermal Properties of Zn/Al-Layered Double Hydroxide Nanocomposite Intercalated with Sodium Dodecyl Sulfate [J].
Babakhani, Samaneh ;
Talib, Zainal Abidin ;
Hussein, Mohd Zobir ;
Ahmed, Abdullah Ahmed Ali .
JOURNAL OF SPECTROSCOPY, 2014, 2014 :1-10
[5]   Bioaugmentation and Adsorption Treatment of Coking Wastewater Containing Pyridine and Quinoline Using Zeolite-Biological Aerated Filters [J].
Bai, Yaohui ;
Sun, Qinghua ;
Sun, Renhua ;
Wen, Donghui ;
Tang, Xiaoyan .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2011, 45 (05) :1940-1948
[6]   POLYTYPE DIVERSITY OF THE HYDROTALCITE-LIKE MINERALS .2. DETERMINATION OF THE POLYTYPES OF EXPERIMENTALLY STUDIED VARIETIES [J].
BOOKIN, AS ;
CHERKASHIN, VI ;
DRITS, VA .
CLAYS AND CLAY MINERALS, 1993, 41 (05) :558-564
[7]   Study on the intercalation of hexacyanoferrate(II) in a Ni, Al based hydrotalcite [J].
Carpani, I ;
Berrettoni, M ;
Ballarin, B ;
Giorgetti, M ;
Scavetta, E ;
Tonelli, D .
SOLID STATE IONICS, 2004, 168 (1-2) :167-175
[8]   Adsorption of tannic acid, humic acid, and dyes from water using the composite of chitosan and activated clay [J].
Chang, MY ;
Juang, RS .
JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2004, 278 (01) :18-25
[9]   Removal of 2-chlorophenol from aqueous solution by Mg/Al layered double hydroxide (LDH) and modified LDH [J].
Chuang, Ya Hui ;
Tzou, Yu Min ;
Wang, Ming Kuang ;
Liu, Cheng Hua ;
Chiang, Po Neng .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2008, 47 (11) :3813-3819
[10]   Structural aspects of layered double hydroxides [J].
Evans, DG ;
Slade, RCT .
LAYERED DOUBLE HYDROXIDES, 2006, 119 :1-87