Broadband Doppler-limited two-photon and stepwise excitation spectroscopy with laser frequency combs

被引:42
作者
Hipke, Arthur [1 ,2 ]
Meek, Samuel A. [2 ]
Ideguchi, Takuro [2 ]
Haensch, Theodor W. [1 ,2 ]
Picque, Nathalie [1 ,2 ,3 ]
机构
[1] Univ Munich, Fak Phys, D-80799 Munich, Germany
[2] Max Planck Inst Quantenoptik, D-85748 Garching, Germany
[3] Univ Paris Sud, CNRS, Inst Sci Mol Orsay, F-91405 Orsay, France
基金
欧洲研究理事会;
关键词
SPECTRA;
D O I
10.1103/PhysRevA.90.011805
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Multiplex two-photon excitation spectroscopy is demonstrated at Doppler-limited resolution. We describe first Fourier-transform two-photon spectroscopy of an atomic sample with two mode-locked laser oscillators in a dual-comb technique. Each transition is uniquely identified by the modulation imparted by the interfering comb excitations. The temporal modulation of the spontaneous two-photon fluorescence is monitored with a single photodetector, and the spectrum of all excited transitions is revealed by a Fourier transform.
引用
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页数:5
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