Effect of Au Precursor and Support on the Catalytic Activity of the Nano-Au-Catalysts for Propane Complete Oxidation

被引:12
|
作者
Ali, Arshid M. [1 ]
Daous, Muhammad A. [1 ]
Arafat, Ahmed [1 ]
AlZahrani, Abdulraheem A. [1 ]
Alhamed, Yahia [1 ]
Tuerdimaimaiti, Abudula [1 ]
Petrov, Lachezar A. [2 ]
机构
[1] King Abdulaziz Univ, Fac Engn, Dept Chem & Mat Engn, Jeddah 21589, Saudi Arabia
[2] King Abdulaziz Univ, SABIC Chair Catalysis, Jeddah 21589, Saudi Arabia
关键词
PREFERENTIAL CO OXIDATION; GOLD CATALYSTS; CALCINATION TEMPERATURE; CARBON-MONOXIDE; DEPOSITION-PRECIPITATION; TIO2; TITANIA; NANOPARTICLES; OXIDES; MECHANISM;
D O I
10.1155/2015/901439
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Catalytic activity of nano-Au-catalyst(s) for the complete propane oxidation was investigated. The results showed that the nature of both Au precursor and support strongly influences catalytic activity of the Au-catalyst(s) for the propane oxidation. Oxidation state, size, and dispersion of Au nanoparticles in the Au-catalysts, surface area, crystallinity, phase structure, and redox property of the support are the key aspects for the complete propane oxidation. Among the studied Au-catalysts, the Au-HAuCl4-Ce catalyst is found to be the most active catalyst.
引用
收藏
页数:10
相关论文
共 50 条
  • [11] Depletion of CO oxidation activity of supported Au catalysts prepared from thiol-capped Au nanoparticles by sulfates formed at Au-titania boundaries: Effects of heat treatment conditions on catalytic activity
    Tai, Yutaka
    Yamaguchi, Wataru
    Okada, Masahisa
    Ohashi, Fumihiko
    Shimizu, Ken-ichi
    Satsuma, Atsushi
    Tajiri, Koji
    Kageyama, Hiroyuki
    JOURNAL OF CATALYSIS, 2010, 270 (02) : 234 - 241
  • [12] Factors influencing structure and catalytic activity of Au/Ce1-xZrxO2 catalysts in CO oxidation
    Dobrosz-Gomez, Izabela
    Kocemba, Ireneusz
    Rynkowski, Jacek M.
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2009, 88 (1-2) : 83 - 97
  • [13] Preparation and Enhanced Catalytic Activity of Pt-Au Alloy Catalysts for Formic Acid Oxidation
    Guo, Chunmei
    Zhang, Mingxing
    Tian, Huifeng
    Wang, Tong
    Hu, Jingbo
    JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2013, 160 (11) : F1187 - F1191
  • [14] Preparation of Au/Ti-SBA-15 Catalysts and Their Catalytic Performance for CO Oxidation
    Su Jixin
    Ma Liyuan
    Zhang Shenping
    Yin Jing
    Qu Wen
    Ding Yi
    CHINESE JOURNAL OF CATALYSIS, 2009, 30 (07) : 659 - 665
  • [15] Catalytic and noncatalytic CO oxidation on Au/TiO2 catalysts
    Soares, JMC
    Morrall, P
    Crossley, A
    Harris, P
    Bowker, M
    JOURNAL OF CATALYSIS, 2003, 219 (01) : 17 - 24
  • [16] Bimetallic Au-Ag catalysts in HCHO catalytic oxidation: No synergetic effect?
    Chen, Dan
    He, Xiuzi
    Chen, Xin
    Wang, Zhong
    Wang, Xiaozhi
    SEPARATION AND PURIFICATION TECHNOLOGY, 2022, 301
  • [17] Preferential Oxidation of CO in H2 Stream on Au/TiO2 Catalysts: Effect of Preparation Method
    Sangeetha, Palanivelu
    Chang, Li-Hsin
    Chen, Yu-Wen
    INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2009, 48 (12) : 5666 - 5670
  • [18] Effect of MgO content in the support of Au/MgF2-MgO catalysts on CO oxidation
    Tomska-Foralewska, Iwona
    Przystajko, Wieslaw
    Pietrowski, Mariusz
    Zielinski, Michal
    Wojciechowska, Maria
    REACTION KINETICS MECHANISMS AND CATALYSIS, 2010, 100 (01) : 111 - 121
  • [19] Effect of the oxidation state of gold on the complete oxidation of isobutane on Au/CeO2 catalysts
    Ying, Fang
    Wang, Shuiju
    Au, Chak-Tong
    Lai, Suk-Yin
    GOLD BULLETIN, 2010, 43 (04): : 241 - 251
  • [20] CO and VOCs Catalytic Oxidation Over Alumina Supported Cu-Mn Catalysts: Effect of Au or Ag Deposition
    Tabakova, T.
    Kolentsova, E.
    Dimitrov, D.
    Ivanov, K.
    Manzoli, M.
    Venezia, A. M.
    Karakirova, Y.
    Petrova, P.
    Nihtianova, D.
    Avdeev, G.
    TOPICS IN CATALYSIS, 2017, 60 (1-2) : 110 - 122