Effect of Au Precursor and Support on the Catalytic Activity of the Nano-Au-Catalysts for Propane Complete Oxidation

被引:13
作者
Ali, Arshid M. [1 ]
Daous, Muhammad A. [1 ]
Arafat, Ahmed [1 ]
AlZahrani, Abdulraheem A. [1 ]
Alhamed, Yahia [1 ]
Tuerdimaimaiti, Abudula [1 ]
Petrov, Lachezar A. [2 ]
机构
[1] King Abdulaziz Univ, Fac Engn, Dept Chem & Mat Engn, Jeddah 21589, Saudi Arabia
[2] King Abdulaziz Univ, SABIC Chair Catalysis, Jeddah 21589, Saudi Arabia
关键词
PREFERENTIAL CO OXIDATION; GOLD CATALYSTS; CALCINATION TEMPERATURE; CARBON-MONOXIDE; DEPOSITION-PRECIPITATION; TIO2; TITANIA; NANOPARTICLES; OXIDES; MECHANISM;
D O I
10.1155/2015/901439
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Catalytic activity of nano-Au-catalyst(s) for the complete propane oxidation was investigated. The results showed that the nature of both Au precursor and support strongly influences catalytic activity of the Au-catalyst(s) for the propane oxidation. Oxidation state, size, and dispersion of Au nanoparticles in the Au-catalysts, surface area, crystallinity, phase structure, and redox property of the support are the key aspects for the complete propane oxidation. Among the studied Au-catalysts, the Au-HAuCl4-Ce catalyst is found to be the most active catalyst.
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页数:10
相关论文
共 64 条
[1]  
Ali A. M., 2014, APPL CATAL A-GEN, V489, P24
[2]   The revision of the air quality legislation in the European Union related to ground-level ozone [J].
Amann, M ;
Lutz, M .
JOURNAL OF HAZARDOUS MATERIALS, 2000, 78 (1-3) :41-62
[3]   The influence of the preparation methods on the catalytic activity of platinum and gold supported on TiO2 for CO oxidation [J].
Bamwenda, GR ;
Tsubota, S ;
Nakamura, T ;
Haruta, M .
CATALYSIS LETTERS, 1997, 44 (1-2) :83-87
[4]   Pd- and/or Au-Loaded Nb- and V-Doped Macro-Mesoporous TiO2 Supports as Catalysts for the Total Oxidation of VOCs [J].
Barakat, Tarek ;
Rooke, Joanna C. ;
Franco, Manuel ;
Cousin, Renaud ;
Lamonier, Jean-Francois ;
Giraudon, Jean-Marc ;
Su, Bao-Lian ;
Siffert, Stephane .
EUROPEAN JOURNAL OF INORGANIC CHEMISTRY, 2012, (16) :2812-2818
[5]   Au/TiO2 nanosized samples:: A catalytic, TEM, and FTIR study of the effect of calcination temperature on the CO oxidation [J].
Boccuzzi, F ;
Chiorino, A ;
Manzoli, M ;
Lu, P ;
Akita, T ;
Ichikawa, S ;
Haruta, M .
JOURNAL OF CATALYSIS, 2001, 202 (02) :256-267
[6]  
Bond G.C., 2006, CATALYSIS GOLD, DOI [10.1007/bf03215560, DOI 10.1007/BF03215560]
[7]   Catalysis by gold [J].
Bond, GC ;
Thompson, DT .
CATALYSIS REVIEWS-SCIENCE AND ENGINEERING, 1999, 41 (3-4) :319-388
[8]   Gold: a relatively new catalyst [J].
Bond, GC .
CATALYSIS TODAY, 2002, 72 (1-2) :5-9
[9]   Exotemplated ceria catalysts with gold for CO oxidation [J].
Carabineiro, S. A. C. ;
Bastos, S. S. T. ;
Orfao, J. J. M. ;
Pereira, M. F. R. ;
Delgado, J. L. ;
Figueiredo, J. L. .
APPLIED CATALYSIS A-GENERAL, 2010, 381 (1-2) :150-160
[10]   Nanocrystalline CeO2 increases the activity of an for CO oxidation by two orders of magnitude [J].
Carrettin, S ;
Concepción, P ;
Corma, A ;
Nieto, JML ;
Puntes, VF .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2004, 43 (19) :2538-2540