Ultrasonic irradiation-induced degradation of low-concentration bisphenol A in aqueous solution

被引：67

作者：

Guo, Zhaobing ^{[1
]}

Feng, Ruo ^{[2
]}

机构：

[1] Nanjing Univ Informat Sci & Technol, Sch Environm Sci & Engn, Nanjing 210044, Peoples R China

[2] Nanjing Univ, Inst Acoust, Nanjing 210093, Peoples R China

来源：

JOURNAL OF HAZARDOUS MATERIALS | 2009年 / 163卷 / 2-3期

关键词：

Bisphenol A; Ultrasonic degradation; Degradation pathway; INDUCED OXIDATION; WATER; PARAMETERS; KINETICS; CAVITATION; SONOLYSIS;

D O I：

10.1016/j.jhazmat.2008.07.038

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

The treatment of bisphenol A (BPA)-contaminated water has attracted great interest recently. In this contribution, ultrasound (US) was applied to remove low-concentration BPA in aqueous solution at the frequency of 20 kHz, and the effects of ultrasonic intensity and ozone on BPA removal were evaluated for the first time. Considering the coexistence of halomethanes and BPA in chlorinated drinking water, BPA was degraded under US in the presence of CCl4, In addition, the main intermediates resulting from BPA ultrasonic degradation were identified by gas chromatography-mass spectrometry. On the basis of these studies, (OH)-O-center dot radical induced oxidation was identified as the major destruction pathway during BPA sonolysis. (C) 2008 Elsevier B.V. All rights reserved.

引用

页码：855 / 860

页数：6

共 30 条

[1] Sonochemistry in environmental remediation. 1. Combinative and hybrid sonophotochemical oxidation processes for the treatment of pollutants in water [J].

Adewuyi, YG .

ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2005, 39 (10) :3409-3420

[2] Kinetics of aqueous ozone-induced oxidation of some endocrine disruptors [J].

Deborde, M ;

Rabouan, S ;

Duguet, JP ;

Legube, B .

ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2005, 39 (16) :6086-6092

[3] Wastewater pretreatment with ultrasonic irradiation to reduce toxicity [J].

Gonze, E ;

Fourel, L ;

Gonthier, Y ;

Boldo, P ;

Bernis, A .

CHEMICAL ENGINEERING JOURNAL, 1999, 73 (02) :93-100

[4] Effect of various sono-oxidation parameters on the removal of aqueous 2,4-dinitrophenol [J].

Guo, ZB ;

Zheng, Z ;

Zheng, SR ;

Hu, WY ;

Feng, R .

ULTRASONICS SONOCHEMISTRY, 2005, 12 (06) :461-465

[5] Improvement in properties of coal water slurry by combined use of new additive and ultrasonic irradiation [J].

Guo, Zhaobing ;

Feng, Ruo ;

Zheng, Youfei ;

Fu, Xiaoru .

ULTRASONICS SONOCHEMISTRY, 2007, 14 (05) :583-588

[6] Sonodegradation of halomethane mixtures in chlorinated drinking water [J].

Guo, Zhaobing ;

Gu, Chunhui ;

Zheng, Zheng ;

Feng, Ruo ;

Jiang, Fang ;

Gao, Guizhi ;

Zheng, Youfei .

ULTRASONICS SONOCHEMISTRY, 2006, 13 (06) :487-492

[7] Products of aqueous chlorination of bisphenol A and their estrogenic activity [J].

Hu, JY ;

Aizawa, T ;

Ookubo, S .

ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2002, 36 (09) :1980-1987

[8] Biodegradation of bisphenol A in the aquatic environment [J].

Ike, M ;

Jin, CS ;

Fujita, M .

WATER SCIENCE AND TECHNOLOGY, 2000, 42 (7-8) :31-38

[9] Impacts of pH and molecular structure on ultrasonic degradation of azo dyes [J].

Ince, NH ;

Tezcanli-Güyer, G .

ULTRASONICS, 2004, 42 (1-9) :591-596

[10] Reactive dyestuff degradation by combined sonolysis and ozonation [J].

Ince, NH ;

Tezcanlí, G .

DYES AND PIGMENTS, 2001, 49 (03) :145-153

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