A self-reinforcing and self-healing elastomer with high strength, unprecedented toughness and room-temperature reparability

被引:253
作者
Li, Yuhan [1 ,2 ]
Li, Wenjuan [1 ,2 ]
Sun, Ailing [1 ,2 ]
Jing, Mengfan [3 ]
Liu, Xingjiang [1 ,2 ]
Wei, Liuhe [1 ,2 ]
Wu, Kai [4 ]
Fu, Qiang [4 ]
机构
[1] Zhengzhou Univ, Coll Chem, Zhengzhou Key Lab Elast Sealing Mat, Zhengzhou 450001, Peoples R China
[2] Zhengzhou Univ, Green Catalysis Ctr, Zhengzhou Key Lab Elast Sealing Mat, Zhengzhou 450001, Peoples R China
[3] Zhengzhou Univ, Natl Engn Res Ctr Adv Polymer Proc Technol, Key Lab Mat Proc & Mold, Zhengzhou 450001, Peoples R China
[4] Sichuan Univ, State Key Lab Polymer Mat & Engn, Coll Polymer Sci & Engn, Chengdu 610065, Peoples R China
基金
中国国家自然科学基金;
关键词
BONDS;
D O I
10.1039/d0mh01447h
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The development of intrinsic self-healing elastomers with simultaneous high mechanical strength, toughness and room-temperature reparability remains a formidable challenge. Herein, we report a mechano-responsive strategy, known as strain induced crystallization, to address the above issue, whereby synthesized elastomers with unprecedented high mechanical performances are bestowed with room-temperature self-healing materials, achieving tensile strength, toughness and fracture energy values of 29.0 MPa, 121.8 MJ m(-3) and 104.1 kJ m(-2), respectively.
引用
收藏
页码:267 / 275
页数:9
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