A versatile prototype plasma reactor for water treatment supporting different discharge regimes

被引:15
作者
Ceriani, Elisa [1 ]
Marotta, Ester [1 ]
Schiorlin, Milko [1 ,3 ]
Ren, Xianwen [1 ,4 ]
Ceretta, Claudio [2 ]
Gobbo, Renato [2 ]
Tampieri, Francesco [1 ]
Paradisi, Cristina [1 ]
机构
[1] Univ Padua, Dept Chem Sci, Via Marzolo 1, I-35131 Padua, Italy
[2] Univ Padua, Dept Ind Engn, Via Gradenigo 6, I-35131 Padua, Italy
[3] Leibniz Inst Plasma Sci & Technol INP Greifswald, Felix Hausdorff Str 2, D-17489 Greifswald, Germany
[4] China Acad Engn Phys, Inst Environm Protect Engn, POB 919-826, Mianyang 621900, Peoples R China
关键词
phenol; nitrophenol; DC discharge; DBD; scaling up; AIR NONTHERMAL PLASMA; ADVANCED OXIDATION; POLLUTION CONTROL; ORGANIC-COMPOUNDS; PHENOL; REMOVAL; REMEDIATION; IONS;
D O I
10.1088/1361-6463/aac7cd
中图分类号
O59 [应用物理学];
学科分类号
摘要
A comparative evaluation is reported of the performance of different discharge regimes-AC powered dielectric barrier discharge (DBD) and DC powered corona discharge of positive (DC+) and negative (DC-) polarity-implemented within the same reactor, a benchtop prototype for an advanced oxidation stage in water treatment. For all three modes of operation, DBD, DC+ and DC-, the reactor performance was tested using phenol as model pollutant and determining the process energy efficiency (k(E) and G(50)), kinetics (t(1/2)), nitrated byproducts and extent of mineralization to CO2. Finally, comparison with a smaller DBD reactor of similar configuration previously used in our lab (Marotta et al 2011 Plasma Proc. Polym. 8 867) shows that scaling up was carried out successfully and holds promise for larger scale applications.
引用
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页数:13
相关论文
共 44 条
[1]   Comparative study between laboratory and large pilot scales for VOC's removal from gas streams in continuous flow surface discharge plasma [J].
Assadi, Aymen Amine ;
Bouzaza, Abdelkrim ;
Wolbert, Dominique .
CHEMICAL ENGINEERING RESEARCH & DESIGN, 2016, 106 :308-314
[2]   A review on catalytic applications of Au/TiO2 nanoparticles in the removal of water pollutant [J].
Ayati, Ali ;
Ahmadpour, Ali ;
Bamoharram, Fatemeh F. ;
Tanhaei, Bahareh ;
Manttari, Mika ;
Sillanpaa, Mika .
CHEMOSPHERE, 2014, 107 :163-174
[3]   MOBILITIES OF SEVERAL MASS-IDENTIFIED POSITIVE AND NEGATIVE-IONS IN AIR [J].
BOHRINGER, H ;
FAHEY, DW ;
LINDINGER, W ;
HOWORKA, F ;
FEHSENFELD, FC ;
ALBRITTON, DL .
INTERNATIONAL JOURNAL OF MASS SPECTROMETRY AND ION PROCESSES, 1987, 81 :45-65
[4]   Characterization and comparative evaluation of two atmospheric plasma sources for water treatment [J].
Bosi, Franco J. ;
Tampieri, Francesco ;
Marotta, Ester ;
Bertani, Roberta ;
Pavarin, Daniele ;
Paradisi, Cristina .
PLASMA PROCESSES AND POLYMERS, 2018, 15 (03)
[5]   Plasma-liquid interactions: a review and roadmap [J].
Bruggeman, P. J. ;
Kushner, M. J. ;
Locke, B. R. ;
Gardeniers, J. G. E. ;
Graham, W. G. ;
Graves, D. B. ;
Hofman-Caris, R. C. H. M. ;
Maric, D. ;
Reid, J. P. ;
Ceriani, E. ;
Rivas, D. Fernandez ;
Foster, J. E. ;
Garrick, S. C. ;
Gorbanev, Y. ;
Hamaguchi, S. ;
Iza, F. ;
Jablonowski, H. ;
Klimova, E. ;
Kolb, J. ;
Krcma, F. ;
Lukes, P. ;
Machala, Z. ;
Marinov, I. ;
Mariotti, D. ;
Thagard, S. Mededovic ;
Minakata, D. ;
Neyts, E. C. ;
Pawlat, J. ;
Petrovic, Z. Lj ;
Pflieger, R. ;
Reuter, S. ;
Schram, D. C. ;
Schroter, S. ;
Shiraiwa, M. ;
Tarabova, B. ;
Tsai, P. A. ;
Verlet, J. R. R. ;
von Woedtke, T. ;
Wilson, K. R. ;
Yasui, K. ;
Zvereva, G. .
PLASMA SOURCES SCIENCE & TECHNOLOGY, 2016, 25 (05)
[6]  
Centi G., 2014, Handbook of Advanced Methods And Processes in Oxidation Catalysis, P251
[7]   Complete mineralization of organic pollutants in water by treatment with air non-thermal plasma [J].
Ceriani, Elisa ;
Marotta, Ester ;
Shapoval, Volodymyr ;
Favaro, Gabriella ;
Paradisi, Cristina .
CHEMICAL ENGINEERING JOURNAL, 2018, 337 :567-575
[8]  
Creijghton Y L M, 1998, Patent US, Patent No. 19960768475
[9]  
Denes F, 2004, Patent US, Patent No. 20020194751
[10]   Plasma-based water purification: Challenges and prospects for the future [J].
Foster, John E. .
PHYSICS OF PLASMAS, 2017, 24 (05)