Electron Transfer-Based Single Molecule Fluorescence as a Probe for Nano-Environment Dynamics

被引:12
作者
Chen, Ruiyun [1 ]
Wu, Ruixiang [1 ]
Zhang, Guofeng [1 ]
Gao, Yan [1 ]
Xiao, Liantuan [1 ]
Jia, Suotang [1 ]
机构
[1] Shanxi Univ, Inst Laser Spect, State Key Lab Quantum Opt & Quantum Opt Devices, Taiyuan 030006, Peoples R China
来源
SENSORS | 2014年 / 14卷 / 02期
基金
对外科技合作项目(国际科技项目);
关键词
single-molecule probes; electron transfer; dynamics; nano-environments; CONJUGATED POLYMER-MOLECULES; ROOM-TEMPERATURE; SOLAR-CELLS; MEH-PPV; PHOTOLUMINESCENCE INTENSITY; HETEROGENEOUS DYNAMICS; LIFETIME FLUCTUATIONS; POLY(VINYL ALCOHOL); SPECTRAL DIFFUSION; ANTHRACENE CRYSTAL;
D O I
10.3390/s140202449
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
Electron transfer (ET) is one of the most important elementary processes that takes place in fundamental aspects of biology, chemistry, and physics. In this review, we discuss recent research on single molecule probes based on ET. We review some applications, including the dynamics of glass-forming systems, surface binding events, interfacial ET on semiconductors, and the external field-induced dynamics of polymers. All these examples show that the ET-induced changes of fluorescence trajectory and lifetime of single molecules can be used to sensitively probe the surrounding nano-environments.
引用
收藏
页码:2449 / 2467
页数:19
相关论文
共 50 条
  • [31] Theory of the energy transfer efficiency and fluorescence lifetime distribution in single-molecule FRET
    Gopich, Irina V.
    Szabo, Attila
    [J]. PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2012, 109 (20) : 7747 - 7752
  • [32] Time-Resolved Photoelectron Spectroscopy to Probe Ultrafast Charge Transfer and Electron Dynamics in Solid Surface Systems and at Metal-Molecule Interfaces
    Castiglioni, Luca
    Greif, Michael
    Leuenberger, Dominik
    Roth, Silvan
    Osterwalder, Juerg
    Hengsberger, Matthias
    [J]. CHIMIA, 2011, 65 (05) : 342 - 345
  • [33] Quantitative monitoring of 2-oxoglutarate in Escherichia coli cells by a fluorescence resonance energy transfer-based biosensor
    Zhang, Chang
    Wei, Zi-Han
    Ye, Bang-Ce
    [J]. APPLIED MICROBIOLOGY AND BIOTECHNOLOGY, 2013, 97 (18) : 8307 - 8316
  • [34] Manifestation of tunneling TLS dynamics of a polymer matrix in single-molecule fluorescence blinking
    S. V. Orlov
    A. V. Naumov
    [J]. Bulletin of the Russian Academy of Sciences: Physics, 2014, 78 (3) : 184 - 188
  • [35] Modelling the Effect of Contact Formation on Electron Transfer in Single-Molecule Device
    Ramos, Marta M. D.
    Correia, Helena M. G.
    [J]. JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY, 2010, 10 (04) : 2570 - 2573
  • [36] Fully Quantized Electron Transfer Observed in a Single Redox Molecule at a Metal Interface
    Roy-Gobeil, Antoine
    Miyahara, Yoichi
    Bevan, Kirk H.
    Grutter, Peter
    [J]. NANO LETTERS, 2019, 19 (09) : 6104 - 6108
  • [37] Single-molecule Conductance and Electrochemical Measurements of Electron Transfer in β-strand Peptides
    Mo, Wenjing
    Horsley, John R.
    Li, Xiaohui
    Sheng, Shiqi
    Jong, Bianca
    Abell, Andrew D.
    Hong, Wenjing
    Yu, Jingxian
    [J]. CHEMELECTROCHEM, 2024, 11 (01)
  • [38] Electron transfer-based peroxydisulfate activation by waste herb residue biochar: Adsorption versus surface oxidation
    Chen, Xuantong
    Guo, Zhen
    Liu, Juemiao
    Wu, Fei
    Cheng, Cheng
    Lin, Heng
    Ren, Wei
    Zhang, Hui
    [J]. CHEMICAL ENGINEERING JOURNAL, 2023, 451
  • [39] Single-molecule fluorescence dynamics of a butadiyne-linked porphyrin dimer: the effect of conformational flexibility in host polymers
    Lee, Ji-Eun
    Yang, Jaesung
    Kim, Dongho
    [J]. FARADAY DISCUSSIONS, 2012, 155 : 277 - 288
  • [40] Charge transfer dynamics from adsorbates to surfaces with single active electron and configuration interaction based approaches
    Ramakrishnan, Raghunathan
    Nest, Mathias
    [J]. CHEMICAL PHYSICS, 2015, 446 : 24 - 29