Silver Nanowire-Modified Filter with Controllable Silver Ion Release for Point-of-Use Disinfection

被引:30
作者
Chen, Wensi [1 ]
Jiang, Jinyue [1 ,2 ]
Zhang, Wenlong [1 ]
Wang, Ting [1 ]
Zhou, Jianfeng [1 ]
Huang, Ching-Hua [1 ]
Xie, Xing [1 ]
机构
[1] Georgia Inst Technol, Sch Civil & Environm Engn, Atlanta, GA 30332 USA
[2] Tsinghua Univ, Sch Environm, Beijing 100084, Peoples R China
关键词
RAPID WATER DISINFECTION; POLYOL SYNTHESIS; ESCHERICHIA-COLI; HIGH-EFFICIENCY; DRINKING-WATER; NANOPARTICLES; COMPOSITE; DISSOLUTION; PERFORMANCE; MECHANISM;
D O I
10.1021/acs.est.9b01678
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Waterborne diseases related to unsafe water are still major threats to public health in some developing countries and rural areas. Providing affordable and safe drinking water globally remains a great challenge in the coming decades. In this study, we develop a high-throughput and conductive silver nanowire (AgNW)-modified composite filter via depositing thin and ultralong AgNWs on a macroporous substrate. An electrochemical filtration cell (EFC) equipped with the composite filter achieves controllable Ag+ release at a mu g L-1 level and superior bacterial inactivation performance (>6-log inactivation efficiency) with an operation voltage of only 1 V at a high flux of 100 m(3) h(-1) m(-2). Under such operation conditions, each composite filter (effective area: 0.79 cm(2)) can treat at least 750 mL of the bacterial suspension (similar to 10(7) CFU mL(-1) of Escherichia coli) with a low effluent Ag+ concentration below 50 mu g L-1 and almost negligible energy consumption of only similar to 70 J m(-3).
引用
收藏
页码:7504 / 7512
页数:9
相关论文
共 70 条
[1]   Emerging opportunities for nanotechnology to enhance water security [J].
Alvarez, Pedro J. J. ;
Chan, Candace K. ;
Elimelech, Menachem ;
Halas, Naomi J. ;
Villagan, Dino .
NATURE NANOTECHNOLOGY, 2018, 13 (08) :634-641
[2]  
[Anonymous], 2017, SAFELY MANAGED DRINK
[3]  
[Anonymous], 2017, Progress on Drinking Water, Sanitation and Hygiene: 2017 Update and SDG Baselines
[4]   Cytotoxicity and Genotoxicity of Silver Nanoparticles in Human Cells [J].
AshaRani, P. V. ;
Mun, Grace Low Kah ;
Hande, Manoor Prakash ;
Valiyaveettil, Suresh .
ACS NANO, 2009, 3 (02) :279-290
[5]   Fecal Contamination of Drinking-Water in Low- and Middle-Income Countries: A Systematic Review and Meta-Analysis [J].
Bain, Robert ;
Cronk, Ryan ;
Wright, Jim ;
Yang, Hong ;
Slaymaker, Tom ;
Bartram, Jamie .
PLOS MEDICINE, 2014, 11 (05)
[6]   Surveillance for Waterborne Disease Outbreaks Associated with Drinking Water - United States, 2013-2014 [J].
Benedict, Katharine M. ;
Reses, Hannah ;
Vigar, Marissa ;
Roth, David M. ;
Roberts, Virginia A. ;
Mattioli, Mia ;
Cooley, Laura A. ;
Hilborn, Elizabeth D. ;
Wade, Timothy J. ;
Fullerton, Kathleen E. ;
Yoder, Jonathan S. ;
Hill, Vincent R. .
MMWR-MORBIDITY AND MORTALITY WEEKLY REPORT, 2017, 66 (44) :1216-1221
[7]   Silver Nanoparticle Surface Functionalized Alumina Filters for Disinfection of Potable Water [J].
Cabala, Guillermo van Erven ;
Acchar, Wilson .
MATERIALS TODAY-PROCEEDINGS, 2015, 2 (01) :321-330
[8]   Effects of Chloride and Ionic Strength on Physical Morphology, Dissolution, and Bacterial Toxicity of Silver Nanoparticles [J].
Chambers, Bryant A. ;
Afrooz, A. R. M. Nabiul ;
Bae, Sungwoo ;
Aich, Nirupam ;
Katz, Lynn ;
Saleh, Navid B. ;
Kirisits, Mary Jo .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2014, 48 (01) :761-769
[9]   Annealing-free, flexible silver nanowire-polymer composite electrodes via a continuous two-step spray-coating method [J].
Choi, Dong Yun ;
Kang, Hyun Wook ;
Sung, Hyung Jin ;
Kim, Sang Soo .
NANOSCALE, 2013, 5 (03) :977-983
[10]   Degradation mechanisms of silver nanowire electrodes under ultraviolet irradiation and heat treatment [J].
Choo, Dong Chul ;
Kim, Tae Whan .
SCIENTIFIC REPORTS, 2017, 7