Zeeman-Tuned Rotational Level-Crossing Spectroscopy in a Diatomic Free Radical

被引:40
作者
Cahn, S. B. [1 ]
Ammon, J. [1 ]
Kirilov, E. [1 ]
Gurevich, Y. V. [1 ]
Murphree, D. [1 ]
Paolino, R. [2 ]
Rahmlow, D. A. [1 ]
Kozlov, M. G. [3 ]
DeMille, D. [1 ]
机构
[1] Yale Univ, Dept Phys, New Haven, CT 06520 USA
[2] US Coast Guard Acad, Dept Sci, New London, CT 06320 USA
[3] Petersburg Nucl Phys Inst, Gatchina 188300, Russia
基金
美国国家科学基金会;
关键词
PARITY NONCONSERVATION; HYPERFINE-STRUCTURE; BAF; MOLECULES; CONSTANTS; SPECTRUM; MOMENTS; DIPOLE;
D O I
10.1103/PhysRevLett.112.163002
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Rotational levels of molecular free radicals can be tuned to degeneracy by using laboratory-scale magnetic fields. Because of their intrinsically narrow width, these level crossings of opposite-parity states have been proposed for use in the study of parity-violating interactions and other applications. We experimentally study a typical manifestation of this system using (BaF)-Ba-138. Using a Stark-mixing method for detection, we demonstrate level-crossing signals with spectral width as small as 6 kHz. We use our data to verify the predicted line shapes, transition dipole moments, and Stark shifts and to precisely determine molecular magnetic g factors. Our results constitute an initial proof of concept for use of this system to study nuclear spin-dependent parity-violating effects.
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页数:5
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