Ozone air quality during the 2008 Beijing Olympics: effectiveness of emission restrictions

被引:148
作者
Wang, Y. [1 ,2 ,3 ,4 ]
Hao, J. [1 ,2 ]
McElroy, M. B. [3 ,4 ]
Munger, J. W. [3 ,4 ]
Ma, H. [1 ,2 ]
Chen, D. [1 ,2 ]
Nielsen, C. P. [4 ,5 ]
机构
[1] Tsinghua Univ, Dept Environm Sci & Engn, Beijing 100084, Peoples R China
[2] Tsinghua Univ, State Key Joint Lab Environm Simulat & Pollut, Beijing 100084, Peoples R China
[3] Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USA
[4] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA
[5] Harvard Univ, Harvard China Project, Cambridge, MA 02138 USA
基金
美国国家科学基金会;
关键词
NITROGEN-OXIDES; CHINA; MODEL; SENSITIVITY; METEOROLOGY; POLLUTANTS; POLLUTION; EXAMPLES; CO;
D O I
10.5194/acp-9-5237-2009
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A series of aggressive measures was launched by the Chinese government to reduce pollutant emissions from Beijing and surrounding areas during the Olympic Games. Observations at Miyun, a rural site 100 km downwind of the Beijing urban center, show significant decreases in concentrations of O-3, CO, NOy, and SO2 during August 2008, relative to August 2006-2007. The mean daytime mixing ratio of O-3 was lower by about 15 ppbv, reduced to 50 ppbv, in August 2008. The relative reductions in daytime SO2, CO, and NOy were 61%, 25%, and 21%, respectively. Changes in SO2 and in species correlations from 2007 to 2008 indicate that emissions of SO2, CO, and NOx were reduced at least by 60%, 32%, and 36%, respectively, during the Olympics. Analysis of meteorological conditions and interpretation of observations using a chemical transport model suggest that although the day-to-day variability in ozone is driven mostly by meteorology, the reduction in emissions of ozone precursors associated with the Olympic Games had a significant contribution to the observed decrease in O-3 during August 2008, accounting for 80% of the O-3 reduction for the month as a whole and 45% during the Olympics Period (8-24 August). The model predicts that emission restrictions such as those implemented during the Olympics can affect O-3 far beyond the Beijing urban area, resulting in reductions in boundary layer O-3 of 2-10 ppbv over a large region of the North China Plain and Northeastern China.
引用
收藏
页码:5237 / 5251
页数:15
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