Simultaneous removal of nitric oxide and sulfur dioxide in a biofilter under micro-oxygen thermophilic conditions: Removal performance, competitive relationship and bacterial community structure

被引:21
作者
Sun, Congcong [1 ,2 ]
Yuan, Jianqi [1 ,2 ]
Xu, Hao [1 ,2 ]
Huang, Shaobin [1 ,2 ]
Wen, Xiangyu [1 ,2 ]
Tong, Na [1 ,2 ]
Zhang, Yongqing [1 ,2 ]
机构
[1] South China Univ Technol, Higher Educ Mega Ctr, Sch Environm & Energy, Guangzhou 510006, Guangdong, Peoples R China
[2] Guangdong Prov Key Lab Atmospher Environm & Pollu, Guangzhou 510006, Guangdong, Peoples R China
基金
中国国家自然科学基金;
关键词
Biofilter; Nitric oxide; Sulfur dioxide; Competitive relationship; Microbial community; ELEMENTAL SULFUR; NITROGEN REMOVAL; NITRATE REMOVAL; FLUE-GAS; SIMULTANEOUS DESULFURIZATION; DEGRADATION EFFICIENCY; SULFIDE-OXIDATION; SULFATE-REDUCTION; DISSOLVED-OXYGEN; CARBON SOURCE;
D O I
10.1016/j.biortech.2019.121768
中图分类号
S2 [农业工程];
学科分类号
0828 ;
摘要
The efficiency of a biofilter to simultaneously remove nitric oxide (NO) and sulfur dioxide (SO2) was investigated under thermophilic (48 +/- 2 degrees C) micro-oxygen (3 vol%) conditions. After the start-up stage (Days 0-14), the stable operation period was divided into three stages. SO2 inlet concentration remained 500 mg/m(3) , NO inlet concentrations were 300 mg/m(3) (Days 15-40), 500 mg/m(3) (Days 41-70) and 700 mg/m(3) (Days 71-100). In each stable stage, the removal efficiency of NO and SO2 exceeded 90%, the maximum removal rates of NO and SO2 were 98.08% and 99.61%, respectively. The final products of SO2 were mostly sulphur. Nitrate-reducing bacteria inhibited sulphate-reducing bacteria. Illumina high-throughput sequencing confirmed that the relative abundance of nitrate-reducing bacteria was positively correlated with NO removal efficiency, the relative abundance of sulphate-reducing bacteria was related to the conversion rate of sulphur.
引用
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页数:8
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