Facile Synthesis of Z-Scheme Ag3PO4/Sulfur-Doped g-C3N4 Heterojunction Hybrids with Enhanced Visible Light Photocatalytic Performance

被引：8

作者：

Bai, Jirong ^{[1
]}

Lv, Wenhua ^{[2
]}

Xu, Haiyang ^{[1
]}

Chen, Gang ^{[1
]}

Ni, Zhijiang ^{[1
]}

Wang, Zhilei ^{[1
]}

Qin, Hengfei ^{[2
]}

Zheng, Zheng ^{[1
]}

Li, Xi ^{[1
,3
]}

机构：

[1] Fudan Univ, Dept Environm Sci & Engn, Shanghai 200433, Peoples R China

[2] Jiangsu Univ Technol, Dept Chem & Environm Engn, Changzhou 213001, Peoples R China

[3] Jiaxing Univ, Coll Biol Chem Sci & Engn, Jiaxing 314001, Peoples R China

来源：

JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY | 2019年 / 19卷 / 09期

关键词：

Ag3PO4; Sulfur-Doped g-C3N4; Heterojunction; Photocatalytic Performance; GRAPHITIC CARBON NITRIDE; IN-SITU SYNTHESIS; COMPOSITE PHOTOCATALYSTS; AG3PO4/G-C3N4; COMPOSITE; PHOTOGENERATED CARRIERS; CONTROLLABLE SYNTHESIS; AG3PO4; NANOPARTICLES; HYDROGEN EVOLUTION; CHARGE SEPARATION; DOPED G-C3N4;

D O I：

10.1166/jnn.2019.16561

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Ag3PO4/sulfur-doped g-C3N4 heterojunctions were fabricated by the means of a facile calcination and co-precipitation method. Structural characterization suggested that Ag3PO4 was successfully loaded onto sulfur-doped g-C(3)N(4. )The absorption band edges of sulfur-doped g-C3N4 were shifted to the longer wavelength in comparison with bulk g-C3N4. The Ag3PO4/sulfur-doped g-C3N4 heterojunctions manifested substantially higher visible-light photocatalytic performance as compared with Ag3PO4/bulkg-C3N4. Photoluminescence spectra suggested that the stable Ag3PO4/SGCN heterojunctions could effectively address the electron-hole recombination rate, together with remarkably enhancing the photocatalytic activity. The enhancement of, light absorption and better dispersion in Ag3PO4/sulfur-doped g-C3N4 provide more migration channels, together with posing crucial responsibility for the enhanced photocatalytic performance.

引用

页码：5736 / 5742

页数：7

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