The formation and physical properties of the particle emissions from a natural gas engine

被引:87
作者
Alanen, Jenni [1 ]
Saukko, Erkka [1 ]
Lehtoranta, Kati [2 ]
Murtonen, Timo [2 ]
Timonen, Hilkka [3 ]
Hillamo, Risto [3 ]
Karjalainen, Panu [1 ]
Kuuluvainen, Heino [1 ]
Harra, Juha [1 ]
Keskinen, Jorma [1 ]
Ronkko, Topi [1 ]
机构
[1] Tampere Univ Technol, Dept Phys, FI-33720 Tampere, Finland
[2] VTT Tech Res Ctr Finland, FI-02044 Espoo, Finland
[3] Finnish Meteorol Inst, Atmospher Composit Res, FI-00101 Helsinki, Finland
关键词
Fine particle emission; Particle formation; Natural gas; Internal combustion engine; NUCLEATION MODE PARTICLES; HEAVY-DUTY; CHARGE-DISTRIBUTION; GASEOUS EMISSIONS; AIR-POLLUTION; STEADY-STATE; ROAD DIESEL; AEROSOL; EXHAUST; SOOT;
D O I
10.1016/j.fuel.2015.09.003
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Natural gas engine particle emissions were studied using an old gasoline engine modified to run with natural gas. The tests were steady-state tests performed on two different low loads in an engine dynamometer. Exhaust particle number concentration, size distribution, volatility and electric charge were measured. Exhaust particles were observed to have peak diameters below 10 nm. To get the full picture of particle emissions from natural gas engines, size range 1-5 nm is relevant and important to take into consideration. A particle size magnifier (PSM) was used in this engine application for measuring particles smaller than 3 nm and it proved to be a useful instrument when measuring natural gas engine exhaust particles. It is concluded that the detected particles probably originated from the engine cylinders or their vicinity and grew to detectable sizes in the sampling process because a small fraction of the particles were observed to carry electric charge and the particles did not evaporate totally at 265 degrees C. (C) 2015 Elsevier Ltd. All rights reserved.
引用
收藏
页码:155 / 161
页数:7
相关论文
共 51 条
[1]   High-resolution low-pressure cascade impactor [J].
Arffman, A. ;
Yli-Ojanpera, J. ;
Kalliokoski, J. ;
Harra, J. ;
Pirjola, L. ;
Karjalainen, P. ;
Ronkko, T. ;
Keskinen, J. .
JOURNAL OF AEROSOL SCIENCE, 2014, 78 :97-109
[2]   Effects of long-term exposure to air pollution on natural-cause mortality: an analysis of 22 European cohorts within the multicentre ESCAPE project [J].
Beelen, Rob ;
Raaschou-Nielsen, Ole ;
Stafoggia, Massimo ;
Andersen, Zorana Jovanovic ;
Weinmayr, Gudrun ;
Hoffmann, Barbara ;
Wolf, Kathrin ;
Samoli, Evangelia ;
Fischer, Paul ;
Nieuwenhuijsen, Mark ;
Vineis, Paolo ;
Xun, Wei W. ;
Katsouyanni, Klea ;
Dimakopoulou, Konstantina ;
Oudin, Anna ;
Forsberg, Bertil ;
Modig, Lars ;
Havulinna, Aki S. ;
Lanki, Timo ;
Turunen, Anu ;
Oftedal, Bente ;
Nystad, Wenche ;
Nafstad, Per ;
De Faire, Ulf ;
Pedersen, Nancy L. ;
Ostenson, Claes-Goeran ;
Fratiglioni, Laura ;
Penell, Johanna ;
Korek, Michal ;
Pershagen, Goeran ;
Eriksen, Kirsten Thorup ;
Overvad, Kim ;
Ellermann, Thomas ;
Eeftens, Marloes ;
Peeters, Petra H. ;
Meliefste, Kees ;
Wang, Meng ;
Bueno-de-Mesquita, Bas ;
Sugiri, Dorothea ;
Kraemer, Ursula ;
Heinrich, Joachim ;
de Hoogh, Kees ;
Key, Timothy ;
Peters, Annette ;
Hampel, Regina ;
Concin, Hans ;
Nagel, Gabriele ;
Ineichen, Alex ;
Schaffner, Emmanuel ;
Probst-Hensch, Nicole .
LANCET, 2014, 383 (9919) :785-795
[3]   Air pollution and health [J].
Brunekreef, B ;
Holgate, ST .
LANCET, 2002, 360 (9341) :1233-1242
[4]   THE OPTICAL CHARACTERIZATION OF HIGH-MOLECULAR-MASS CARBONACEOUS STRUCTURES PRODUCED IN PREMIXED LAMINAR FLAMES ACROSS THE SOOT THRESHOLD LIMIT [J].
BUCHTA, C ;
DALESSIO, A ;
DANNA, A ;
GAMBI, G ;
MINUTOLO, P ;
RUSSO, S .
PLANETARY AND SPACE SCIENCE, 1995, 43 (10-11) :1227-1232
[5]   Size, volatility, and effective density of particulate emissions from a homogeneous charge compression ignition engine using compressed natural gas [J].
Bullock, Dallin S. ;
Olfert, Jason S. .
JOURNAL OF AEROSOL SCIENCE, 2014, 75 :1-8
[6]   Separation of volatile and non-volatile aerosol fractions by thermodesorption:: instrumental development and applications [J].
Burtscher, H ;
Baltensperger, U ;
Bukowiecki, N ;
Cohn, P ;
Hüglin, C ;
Mohr, M ;
Matter, U ;
Nyeki, S ;
Schmatloch, V ;
Streit, N ;
Weingartner, E .
JOURNAL OF AEROSOL SCIENCE, 2001, 32 (04) :427-442
[7]   Characterization of Combustion-Generated Carbonaceous Nanoparticles by Size-Dependent Ultraviolet Laser Photoionization [J].
Commodo, Mario ;
Sgro, Lee Anne ;
Minutolo, Patrizia ;
D'Anna, Andrea .
JOURNAL OF PHYSICAL CHEMISTRY A, 2013, 117 (19) :3980-3989
[8]   Combustion-formed nanoparticles [J].
D'Anna, Andrea .
PROCEEDINGS OF THE COMBUSTION INSTITUTE, 2009, 32 :593-613
[9]   Diesel Nucleation Mode Particles: Semivolatile or Solid? [J].
De Filippo, Andrea ;
Maricq, M. Matti .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2008, 42 (21) :7957-7962
[10]  
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