Imprints of the Molecular Electronic Structure in the Photoelectron Spectra of Strong-Field Ionized Asymmetric Triatomic Model Molecules

被引:13
作者
Paul, Matthias
Yue, Lun
Graefe, Stefanie [1 ]
机构
[1] Friedrich Schiller Univ Jena, Inst Phys Chem, Hehnholtzweg 4, D-07743 Jena, Germany
关键词
CIRCULAR-DICHROISM; ANGULAR-DISTRIBUTIONS; SCHRODINGER-EQUATION; IONIZATION; DYNAMICS; PHOTOEMISSION; ABSORPTION;
D O I
10.1103/PhysRevLett.120.233202
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We examine the circular dichroism in the angular distribution of photoelectrons of triatomic model systems ionized by strong-field ionization. Following our recent work on this effect [Paul, Yue, and Grafe, J. Mod. Opt. 64, 1104 (2017)], we demonstrate how the symmetry and electronic structure of the system is imprinted into the photoelectron momentum distribution. We use classical trajectories to reveal the origin of the three folded pattern in the photoelectron momentum distribution, and show how an asymmetric nuclear configuration of the triatomic system effects the photoelectron spectra.
引用
收藏
页数:6
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