Imprints of the Molecular Electronic Structure in the Photoelectron Spectra of Strong-Field Ionized Asymmetric Triatomic Model Molecules

被引:13
作者
Paul, Matthias
Yue, Lun
Graefe, Stefanie [1 ]
机构
[1] Friedrich Schiller Univ Jena, Inst Phys Chem, Hehnholtzweg 4, D-07743 Jena, Germany
关键词
CIRCULAR-DICHROISM; ANGULAR-DISTRIBUTIONS; SCHRODINGER-EQUATION; IONIZATION; DYNAMICS; PHOTOEMISSION; ABSORPTION;
D O I
10.1103/PhysRevLett.120.233202
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We examine the circular dichroism in the angular distribution of photoelectrons of triatomic model systems ionized by strong-field ionization. Following our recent work on this effect [Paul, Yue, and Grafe, J. Mod. Opt. 64, 1104 (2017)], we demonstrate how the symmetry and electronic structure of the system is imprinted into the photoelectron momentum distribution. We use classical trajectories to reveal the origin of the three folded pattern in the photoelectron momentum distribution, and show how an asymmetric nuclear configuration of the triatomic system effects the photoelectron spectra.
引用
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页数:6
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共 55 条
[1]   Site-specific photoemission dynamics of N2O molecules probed by fixed-molecule core-level photoelectron angular distributions [J].
Adachi, J. ;
Ito, K. ;
Yoshii, H. ;
Yamazaki, M. ;
Yagishita, A. ;
Stener, M. ;
Decleva, P. .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2007, 40 (01) :29-47
[2]   Quantum interference in double ionization and fragmentation of C6H6 in intense laser fields -: art. no. 253003 [J].
Bhardwaj, VR ;
Rayner, DM ;
Villenueve, DM ;
Corkum, PB .
PHYSICAL REVIEW LETTERS, 2001, 87 (25) :253003-253003
[3]   Correlated multielectron systems in strong laser fields: A multiconfiguration time-dependent Hartree-Fock approach [J].
Caillat, J ;
Zanghellini, J ;
Kitzler, M ;
Koch, O ;
Kreuzer, W ;
Scrinzi, A .
PHYSICAL REVIEW A, 2005, 71 (01)
[4]   Controlling electron-electron correlation in frustrated double ionization of triatomic molecules with orthogonally polarized two-color laser fields [J].
Chen, A. ;
Kling, M. F. ;
Emmanouilidou, A. .
PHYSICAL REVIEW A, 2017, 96 (03)
[5]   Frustrated double and single ionization in a two-electron triatomic molecule H3+ [J].
Chen, A. ;
Lazarou, C. ;
Price, H. ;
Emmanouilidou, A. .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2016, 49 (23)
[6]   CIRCULAR-DICHROISM OF MOLECULES IN THE CONTINUOUS ABSORPTION REGION [J].
CHEREPKOV, NA .
CHEMICAL PHYSICS LETTERS, 1982, 87 (04) :344-348
[7]   ENERGY AND ANGULAR ELECTRON-SPECTRA FOR THE TUNNEL IONIZATION OF ATOMS BY STRONG LOW-FREQUENCY RADIATION [J].
DELONE, NB ;
KRAINOV, VP .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 1991, 8 (06) :1207-1211
[8]   Strong-field ionization of polar molecules: Stark-shift-corrected strong-field approximation [J].
Dimitrovski, D. ;
Martiny, C. P. J. ;
Madsen, L. B. .
PHYSICAL REVIEW A, 2010, 82 (05)
[9]   Ionization of oriented carbonyl sulfide molecules by intense circularly polarized laser pulses [J].
Dimitrovski, Darko ;
Abu-samha, Mahmoud ;
Madsen, Lars Bojer ;
Filsinger, Frank ;
Meijer, Gerard ;
Kuepper, Jochen ;
Holmegaard, Lotte ;
Kalhoj, Line ;
Nielsen, Jens H. ;
Stapelfeldt, Henrik .
PHYSICAL REVIEW A, 2011, 83 (02)
[10]   Theoretical investigation of alignment-dependent intense-field fragmentation of acetylene [J].
Doblhoff-Dier, Katharina ;
Kitzler, Markus ;
Graefe, Stefanie .
PHYSICAL REVIEW A, 2016, 94 (01)