Thermal response of a field emitter subjected to ultra-fast laser illumination

被引:96
作者
Vurpillot, F. [1 ]
Houard, J. [1 ]
Vella, A. [1 ]
Deconihout, B. [1 ]
机构
[1] Univ Rouen, CNRS, GPM, UMR 6634, F-76801 St Etienne, France
关键词
ATOM-PROBE; ELECTRIC-FIELD; DESORPTION; TEMPERATURE; TIP; EVAPORATION; MICROSCOPY; EMISSION; IONS;
D O I
10.1088/0022-3727/42/12/125502
中图分类号
O59 [应用物理学];
学科分类号
摘要
Using an ultra-fast laser assisted atom probe, the temporal evolution of the temperature of a tungsten field emitter subjected to illumination is studied. The combination of pump probe experiments and evaporation rate measurements is used to estimate the duration of field evaporation, the induced peak temperature and the cooling time. The main conclusion of the measurements is that, despite a significant heating of the tip by the laser pulse, the cooling time is anomalously fast, below 0.5 ns. Hence, thermal effects are considered to play a major role in ion emission in contrast to conclusions of our previous works. It is shown that the really fast anomalous cooling rate can only be related to a confined heating zone at the tip apex smaller than the wavelength of the laser.
引用
收藏
页数:7
相关论文
共 30 条
[1]   AN ATOM-PROBE FOR 3-DIMENSIONAL TOMOGRAPHY [J].
BLAVETTE, D ;
BOSTEL, A ;
SARRAU, JM ;
DECONIHOUT, B ;
MENAND, A .
NATURE, 1993, 363 (6428) :432-435
[2]   STATE-RESOLVED EVIDENCE FOR HOT CARRIER DRIVEN SURFACE-REACTIONS - LASER-INDUCED DESORPTION OF NO FROM PT(111) [J].
BUNTIN, SA ;
RICHTER, LJ ;
KING, DS ;
CAVANAGH, RR .
JOURNAL OF CHEMICAL PHYSICS, 1989, 91 (10) :6429-6446
[3]   Aspects of the performance of a femtosecond laser-pulsed 3-dimensional atom probe [J].
Cerezo, A. ;
Clifton, P. H. ;
Gomberg, A. ;
Smith, G. D. W. .
ULTRAMICROSCOPY, 2007, 107 (09) :720-725
[4]   Measurement of temperature rises in the femtosecond laser pulsed three-dimensional atom probe [J].
Cerezo, A ;
Smith, GDW ;
Clifton, PH .
APPLIED PHYSICS LETTERS, 2006, 88 (15)
[5]   Design of a femtosecond laser assisted tomographic atom probe [J].
Gault, B ;
Vurpillot, F ;
Vella, A ;
Gilbert, M ;
Menand, A ;
Blavette, D ;
Deconihout, B .
REVIEW OF SCIENTIFIC INSTRUMENTS, 2006, 77 (04)
[6]   FIELD DESORPTION [J].
GOMER, R .
JOURNAL OF CHEMICAL PHYSICS, 1959, 31 (02) :341-345
[7]   Photoassisted scanning tunneling microscopy [J].
Grafström, S .
JOURNAL OF APPLIED PHYSICS, 2002, 91 (04) :1717-1753
[8]   Photoelectric field emission from needle cathodes [J].
Hernandez-Garcia, C ;
Brau, CA .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 1999, 429 (1-3) :257-263
[9]   Field emission tip as a nanometer source of free electron femtosecond pulses [J].
Hommelhoff, P ;
Sortais, Y ;
Aghajani-Talesh, A ;
Kasevich, MA .
PHYSICAL REVIEW LETTERS, 2006, 96 (07) :1-4