Time-resolved photoluminescence properties of semiconductor quantum dot superlattices of different microcrystal shapes

被引:6
作者
Chae, Weon-Sik [1 ]
Choi, Eunjin [1 ]
Jung, Yun Ku [1 ]
Jung, Jin-Seung [2 ]
Lee, Jin-Kyu [3 ]
机构
[1] Korea Basic Sci Inst, Kangnung 210702, South Korea
[2] Gangneung Wonju Natl Univ, Dept Chem, Kangnung 210702, South Korea
[3] Seoul Natl Univ, Dept Chem, Seoul 151747, South Korea
基金
新加坡国家研究基金会;
关键词
NANOPARTICLE SUPERLATTICES; NANOCRYSTALS; CDSE; BLINKING;
D O I
10.1063/1.4871468
中图分类号
O59 [应用物理学];
学科分类号
摘要
We report time-resolved photoluminescence properties on semiconductor quantum dot (QD) superlattices (SLs) using PL lifetime imaging microscopy at a single particle level. PL lifetime imaging technique clearly reveals that different shaped QD SL microcrystals have different time-resolved PL characteristics. The faceted SL microcrystals consisted of well-organized QDs showed faster recombination rates than those of the spherical microparticles including randomly organized QDs, which can be explained by the different degree of energetic couplings among component QDs due to different packing fraction. (C) 2014 AIP Publishing LLC.
引用
收藏
页数:3
相关论文
共 28 条
[1]  
BRAUN PV, 2003, NANOCOMPOSITE SCI TE
[2]   Binary nanoparticle superlattices in the semiconductor-semiconductor system: CdTe and CdSe [J].
Chen, Zhuoying ;
Moore, Jenny ;
Radtke, Guillaume ;
Sirringhaus, Henning ;
O'Brien, Stephen .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (50) :15702-15709
[3]   Magnetic superlattices and their nanoscale phase transition effects [J].
Cheon, J ;
Park, JI ;
Choi, JS ;
Jun, YW ;
Kim, S ;
Kim, MG ;
Kim, YM ;
Kim, YJ .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2006, 103 (09) :3023-3027
[4]   Improving the density of jammed disordered packings using ellipsoids [J].
Donev, A ;
Cisse, I ;
Sachs, D ;
Variano, E ;
Stillinger, FH ;
Connelly, R ;
Torquato, S ;
Chaikin, PM .
SCIENCE, 2004, 303 (5660) :990-993
[5]   Model of Fluorescence Intermittency of Single Colloidal Semiconductor Quantum Dots Using Multiple Recombination Centers [J].
Frantsuzov, Pavel A. ;
Volkan-Kacso, Sandor ;
Janko, Boldizsar .
PHYSICAL REVIEW LETTERS, 2009, 103 (20)
[6]   Two types of luminescence blinking revealed by spectroelectrochemistry of single quantum dots [J].
Galland, Christophe ;
Ghosh, Yagnaseni ;
Steinbrueck, Andrea ;
Sykora, Milan ;
Hollingsworth, Jennifer A. ;
Klimov, Victor I. ;
Htoon, Han .
NATURE, 2011, 479 (7372) :203-U75
[7]   Synthesis of monodisperse palladium nanoparticles [J].
Kim, SW ;
Park, J ;
Jang, Y ;
Chung, Y ;
Hwang, S ;
Hyeon, T ;
Kim, YW .
NANO LETTERS, 2003, 3 (09) :1289-1291
[8]   Super-efficient exciton funneling in layer-by-layer semiconductor nanocrystal structures [J].
Klar, TA ;
Franzl, T ;
Rogach, AL ;
Feldmann, J .
ADVANCED MATERIALS, 2005, 17 (06) :769-773
[9]   Comparison of Structural Behavior of Nanocrystals in Randomly Packed Films and Long-Range Ordered Superlattices by Time-Resolved Small Angle X-ray Scattering [J].
Lee, Byeongdu ;
Podsiadlo, Paul ;
Rupich, Sara ;
Talapin, Dmitri V. ;
Rajh, Tijana ;
Shevchenko, Elena V. .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2009, 131 (45) :16386-+
[10]   Face-centered cubic "supracrystals" of cobalt nanocrystals [J].
Lisiecki, I ;
Albouy, PA ;
Pileni, MP .
ADVANCED MATERIALS, 2003, 15 (09) :712-716